Local Liquid Side Mass Transfer Model in Gas-Liquid-Solid Three-Phase Flow Airlift Loop Reactor for Newtonian and Non-Newtonian Fluids  

作　　者：闻建平 贾晓强 毛国柱 

机构地区：[1]Department of Biochemical Engineering, School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, China [2]Department of Biochemical Engineering, School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, China small scale isotropic mass transfer model was developed for the local liquid side mass transfer coefficients in gas-liquid-solid three-phase flow airlift loop reactor for Newtonian and non-Newtonian fluids. It is based onHigbie's penetration theory and Kolmogoroff's theory of isotropic turbulence withwhere ε1 is local rate of energy dissipation, Af is the local microscale, η1 is the local Kolmogoroff scale and D is the diffusion coefficient. The capability of the proposed model is discussed in the light of experimental data obtained from 12 L gas-liquid-solid three-phase flow airlift loop reactor using Newtonian and non-Newtonian fluids. Good agreement with the experimental data was obtained over a wide range of conditions suggesting a general applicability of the proposed model.

出　　处：《Chinese Journal of Chemical Engineering》2004年第3期347-350,共4页中国化学工程学报（英文版）

基　　金：the National Natural Science Foundation of China (No. 20176040, No. 20336030 and No. 90206001).

摘　　要：A small scale isotropic mass transfer model was developed for the local liquid side mass transfer coefficients in gas-liquid-solid three-phase flow airlift loop reactor for Newtonian and non-Newtonian fluids. It is based onHigbie's penetration theory and Kolmogoroff's theory of isotropic turbulence withwhere ε1 is local rate of energy dissipation, Af is the local microscale, η1 is the local Kolmogoroff scale and D is the diffusion coefficient. The capability of the proposed model is discussed in the light of experimental data obtained from 12 L gas-liquid-solid three-phase flow airlift loop reactor using Newtonian and non-Newtonian fluids. Good agreement with the experimental data was obtained over a wide range of conditions suggesting a general applicability of the proposed model.A small scale isotropic mass transfer model was developed for the local liquid side mass transfer coefficients in gas-liquid-solid three-phase flow airlift loop reactor for Newtonian and non-Newtonian fluids. It is based on Higbie's penetration theory and Kolmogoroff's theory of isotropic turbulence with kl=3√2D∈11/3/π(η1^-1/3-λf^-1/3)where e1 is local rate of energy dissipation, Af is the local microscale, r/l is the local Kolmogoroff scale and D is the diffusion coefficient. The capability of the proposed model is discussed in the light of experimental data obtained from 12 L gas-liquid-solid three-phase flow airlift loop reactor using Newtonian and non-Newtonian fluids. Good agreement with the experimental data was obtained over a wide range of conditions suggesting a general applicability of the proposed model.

关 键 词：DIFFUSIVITY energy dissipation Kolmogoroff scale MICROSCALE penetration theory 

分 类 号：TQ021[化学工程]