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作 者:谷芳 刘春江[1] 余黎明[1] 周超凡[1] 袁希钢[1] 余国琮[1]
机构地区:[1]天津大学化工学院化学工程联合国家重点实验室,天津300072
出 处:《高校化学工程学报》2005年第4期438-444,共7页Journal of Chemical Engineering of Chinese Universities
基 金:国家自然科学基金(20206021);天津市自然科学基金(023606711)
摘 要:利用VOF法建立了考虑表面张力动量源项、气液相间摩擦力动量源项以及相间传质源项的CFD计算模型,定量描述了气-液两相逆流降膜传质过程。根据CFD模型,计算了不同液相进口浓度和不同气相流量条件下,异丙醇稀溶液的解吸过程,模拟得到的液相出口浓度与实验数据吻合很好。相界面处的浓度分布表明,随自由表面波动,界面浓度会发生剧烈脉动。液相总传质系数增强因子R的实验值与CFD模拟均表明,即使在很小的传质推动力下R也大于1。由于CFD模型不考虑Rayleigh-B?nard-Maragoni效应,则这种现象,可解释为界面波动对传质增强的结果。这也证明增强界面波动是一种强化传质分离过程的有效途径。A CFD model using the volume of fluid (VOF) method was presented for predicting the mass-transfer process of the two-phase countercurrent falling film, in which the momentum source term including surface tension and interface shear stress and a mass-transfer source term were given. The model was applied to simulate the stripping process of 2-Propanol dilute solution. It is found that the simulated outlet liquid concentrations under different inlet liquid concentrations and various gas flow rates are in good agreement with the experimental data. The simulations also confirm that with free surface waving the interface concentration fluctuate violently. The enhancement factor R from experiment and CFD simulation are both larger than 1, even under the little mass-transfer impetus. Since the Rayleigh-B?nard-Maragoni effect was not considered in the CFD model, the conclusion can be regarded as that in the simulation, the results of the enhancement of the mass-transfer process is caused by fluctuating interfacial waves, which also proves that fluctuating the interfacial waves is an effective means to enhance the separation efficiency.
关 键 词:计算流体力学(CFD) 降膜 两相流 解吸 传质
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