Controlling optical responses through local dielectric resonance in nanometre metallic clusters  

作　　者：陈亮亮 古英 王立金 龚旗煌 

机构地区：[1]State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University, Beijing 100871, China

出　　处：《Chinese Physics B》2007年第1期249-257,共9页中国物理B（英文版）

基　　金：Project supported by the National Natural Science Foundation of China（Grant Nos 10304001, 10334010, 10521002, 10434020, 10328407 and 90501007）.

摘　　要：Optical responses in dilute composites are controlled through the local dielectric resonance of metallic clusters. We consider two located metallic clusters close to each other with admittances ε1 and ε2. Through varying the difference admittance ratio η[= （ε2 - ε0）/（ε1 - ε0）], we find that their optical responses are determined by the local resonance. There is a blueshift of absorption peaks with the increase of η- Simultaneously, it is known that the absorption peaks will be redshifted by enlarging the cluster size. By adjusting the nano-metallic cluster geometry, size and admittances, we can control the positions and intensities of absorption peaks effectively. We have also deduced the effective linear optical responses of three-component composites εe=ε0 （1＋∑^n n=1[（γn1＋ηγn2）/（ε0（s-sn））]） and the sum rule of cross sections：∑^n n=1（γn1＋ηγn2）=Nh1＋Nh2,, where Nh1and Nh2 are the numbers of εl and ε2 bonds along the electric field, respectively. These results may be beneficial to the study of surface plasmon resonances on a nanometre scale.Optical responses in dilute composites are controlled through the local dielectric resonance of metallic clusters. We consider two located metallic clusters close to each other with admittances ε1 and ε2. Through varying the difference admittance ratio η[= （ε2 - ε0）/（ε1 - ε0）], we find that their optical responses are determined by the local resonance. There is a blueshift of absorption peaks with the increase of η- Simultaneously, it is known that the absorption peaks will be redshifted by enlarging the cluster size. By adjusting the nano-metallic cluster geometry, size and admittances, we can control the positions and intensities of absorption peaks effectively. We have also deduced the effective linear optical responses of three-component composites εe=ε0 （1＋∑^n n=1[（γn1＋ηγn2）/（ε0（s-sn））]） and the sum rule of cross sections：∑^n n=1（γn1＋ηγn2）=Nh1＋Nh2,, where Nh1and Nh2 are the numbers of εl and ε2 bonds along the electric field, respectively. These results may be beneficial to the study of surface plasmon resonances on a nanometre scale.

关 键 词：local dielectric resonance effective linear optical response nanometre metallic cluster 

分 类 号：TB383[一般工业技术—材料科学与工程]