Catalytic Decomposition of Toluene Using Various Dielectric Barrier Discharge Reactors  被引量:2

Catalytic Decomposition of Toluene Using Various Dielectric Barrier Discharge Reactors

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作  者:叶代启 黄海保 陈韦丽 曾荣辉 

机构地区:[1]College of Environmental Science and Engineering, South China University of Technology, Guangzhou 510640, China

出  处:《Plasma Science and Technology》2008年第1期89-93,共5页等离子体科学和技术(英文版)

基  金:National Natural Science Foundation of China(No.20577011);Guangdong Provincial Key Scientific and Technological Project(No.2001367,2002254);Guangzhou Municipal Key Scientific and Technological Project(No.2001-Z-016-01)

摘  要:Decomposition of toluene was experimentally investigated with various dielectric barrier discharge (DBD) reactors, such as wire-cylinder, wire-plate and plate-to-plate, combined with multi-metal oxides catalyst (Mn-Ni-Co-Cu-Ox/Al2O3) loaded on the cordierite honeycomb and nickel foam, respectively. The effects of some factors including the residence time, reactor configuration and catalyst, upon the toluene destruction were studied. Results revealed that the use of in-plasma catalysis was more helpful to enhancing the DRE (destruction and removal efficiency) and reducing the O3 formation than that of either post-plasma catalysis or plasma alone. It was demonstrated that the wire-plate reactor was favorable for the oxidation reaction of toluene and the nickel foam-supported catalysts exhibited good activity.Decomposition of toluene was experimentally investigated with various dielectric barrier discharge (DBD) reactors, such as wire-cylinder, wire-plate and plate-to-plate, combined with multi-metal oxides catalyst (Mn-Ni-Co-Cu-Ox/Al2O3) loaded on the cordierite honeycomb and nickel foam, respectively. The effects of some factors including the residence time, reactor configuration and catalyst, upon the toluene destruction were studied. Results revealed that the use of in-plasma catalysis was more helpful to enhancing the DRE (destruction and removal efficiency) and reducing the O3 formation than that of either post-plasma catalysis or plasma alone. It was demonstrated that the wire-plate reactor was favorable for the oxidation reaction of toluene and the nickel foam-supported catalysts exhibited good activity.

关 键 词:non-thermal plasma dielectric barrier discharge CATALYSIS TOLUENE 

分 类 号:O539[理学—等离子体物理]

 

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