机构地区:[1]Department of Natural Resources, College of Environmental Science and Natural Resources, Zhefiang University, Hangzhou 310029, China. [2]China Ministry of Education Key Laboratory of Environmental Remediation and Ecological Health, Zhefiang University, Hangzhou 310029, China [3]Zhejiang Provincial Key Laboratory of Subtropic Soil and Plant Nutrition, Hangzhou 310029, China [4]Ecology and Environment Institute, Ningbo Academy of Agricultural Science, Ningbo 315040, China
出 处:《Journal of Environmental Sciences》2009年第4期429-433,共5页环境科学学报(英文版)
基 金:supported by the National Natural Science Foundation of China (No. 40571070);the National Basic Research Program (973) of China (No.2002CB410807);the Project of Science and Technology of Zhejiang Province (No. 2004C33067)
摘 要:The distribution of different nitrogen forms and their spatial and temporal variations in different pollution types of tributaries or reaches were investigated. Based on the catchments characteristics the tributaries or reaches can be classified into 4 types, including headwater in mountainous areas (type Ⅰ), agricultural non-point source (NPS) pollution in rural areas (type Ⅱ), municipal and industrial pollution in urban areas (type Ⅲ), and combined pollution in main stream (type IV). Water samples were collected monthly from July 2003 to June 2006 in the Cao-E River Basin in Zhejiang, eastern China. The concentrations of NO3^--N, NH4^+ -N, and total nitrogen (TN) were measured. The mean concentrations of NO3^- -N were decreased in the sequence type IV 〉 type Ⅱ〉 type Ⅲ 〉 type Ⅰ, whereas, NH4^+-N, total organic nitrogen (TON), and TN were in the sequence: type Ⅲ〉 type Ⅳ 〉 type Ⅱ〉 type Ⅰ. In headwater and rural reaches, CNO^-2-N was much higher than Crea^+ 4-N. In urban reaches, TON and NH4^+ -N were the main forms, accounting for 54.7% and 32.1% of TN, respectively. In the whole river system, Crea^+ 4--N decreased with increasing distance from cities, and CNo^-3 -N increased with the increasing area of farmland in the catchments. With increased river flow, CNO^-3 N increased and Crea4^+-N decreased in all types of reaches, while the variations of CTON and CTN were different. For TN, the concentration may be decreased with the increase of river flow, but the export load always increased.The distribution of different nitrogen forms and their spatial and temporal variations in different pollution types of tributaries or reaches were investigated. Based on the catchments characteristics the tributaries or reaches can be classified into 4 types, including headwater in mountainous areas (type Ⅰ), agricultural non-point source (NPS) pollution in rural areas (type Ⅱ), municipal and industrial pollution in urban areas (type Ⅲ), and combined pollution in main stream (type IV). Water samples were collected monthly from July 2003 to June 2006 in the Cao-E River Basin in Zhejiang, eastern China. The concentrations of NO3^--N, NH4^+ -N, and total nitrogen (TN) were measured. The mean concentrations of NO3^- -N were decreased in the sequence type IV 〉 type Ⅱ〉 type Ⅲ 〉 type Ⅰ, whereas, NH4^+-N, total organic nitrogen (TON), and TN were in the sequence: type Ⅲ〉 type Ⅳ 〉 type Ⅱ〉 type Ⅰ. In headwater and rural reaches, CNO^-2-N was much higher than Crea^+ 4-N. In urban reaches, TON and NH4^+ -N were the main forms, accounting for 54.7% and 32.1% of TN, respectively. In the whole river system, Crea^+ 4--N decreased with increasing distance from cities, and CNo^-3 -N increased with the increasing area of farmland in the catchments. With increased river flow, CNO^-3 N increased and Crea4^+-N decreased in all types of reaches, while the variations of CTON and CTN were different. For TN, the concentration may be decreased with the increase of river flow, but the export load always increased.
关 键 词:catchment characteristics NITROGEN FORMS spatial and temporal variation Cao-E River Basin
分 类 号:X522.02[环境科学与工程—环境工程] S572[农业科学—烟草工业]
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