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作 者:李云波[1,2] 王玉晓[2] 张学如[2] 杨昆[2] 石光[2] 蒋礼[3] 杨俊义[1] 宋瑛林[1,2]
机构地区:[1]苏州大学物理科学与技术学院,江苏苏州215006 [2]哈尔滨工业大学物理系,黑龙江哈尔滨150001 [3]中国科学院化学研究所有机固体重点实验室,北京100080
出 处:《红外与激光工程》2010年第2期236-240,284,共6页Infrared and Laser Engineering
基 金:国家自然科学基金资助项目(10774109);教育部新世纪优秀人才计划资助项目(NCET-04-0333);黑龙江省杰出青年基金资助项目(JC-04-04)
摘 要:4f相位相干成像系统是最近发展起来的一种利用单脉冲测量材料三阶非线性的技术。当使用这种技术对薄膜材料进行测量时,部分材料经过高光强照射以后会产生伪非线性图像。这里所说的伪非线性图像是指无论在强的或弱的激光光强照射下,被测量样品的实验结果中总是显示出与非线性材料在高光强下显现出的非线性图像相类似的实验图像。基于多种不同材料的薄膜样品的实验结果,对伪非线性图像的形成原因进行了研究。大量实验表明:伪非线性图像是由样品的两种损伤造成的:一种是样品被碳化或破坏(形成一个黑斑),另一种是样品被剥离或漂白(形成一个白斑)。从实验和数值仿真两方面对观点进行了验证。The nonlinear imaging technique with phase object(NIT-PO) is a newly developed one-lasershot technique used to measure the third-order nonlinearity of materials.When NIT-PO is used to measure thin film materials,some of them will generate pseudo nonlinear images after being exposed to high intensity laser.The pseudo nonlinear images here means that whatever the laser intensity is,the experimental results of measured materials always exhibit image patterns similar to the ones of nonlinear sample under high intensity laser.The reasons to form the pseudo nonlinear images were researched in this paper based the experimental results of different kinds of thin film materials.Based on large number of experiments,we consider that the pseudo nonlinear images are induced by two kinds of sample damage: one is the carbonization or destruction(form a black spot),and the other is laser ablation or bleaching(form a white spot).Our points of view were validated by both experiments and numerical simulations.
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