Pu材料γ能谱分析软件CMGA2.0  

CMGA2.0—A Code to Assay Abundances of Plutonium Isotopes With γ-ray Spectrum

作　　者：徐子骏[1] 王思广[1] 

机构地区：[1]北京大学物理学院及核物理与核技术国家重点实验室,北京100871

出　　处：《原子能科学技术》2010年第B09期657-660,共4页Atomic Energy Science and Technology

基　　金：高等学校博士学科点专项科研基金资助项目(20070001008);国家自然科学基金资助项目(10775006;10979010);国家基础科学人才培养基金资助项目(J0730316)

摘　　要：在92～112keV区间内,Pu材料的多通道γ能谱共包含238Pu、239Pu、240Pu、241Pu和241Am自发衰变发出的8条γ射线和29条X射线。CMGA通过分析该区间能谱,可给出样品中Pu同位素丰度。升级后的CMGA(2.0版)对2例样品6次重复测量的能谱进行分析,其给出的240Pu与239Pu含量的比值分别为质谱分析结果的1.010±0.008和0.995±0.011。通过对比CMGA2.0使用不同本底描述方法得到的92～105keV区间能谱拟合图,可看出双线性积分步本底函数可更好地描述复杂重峰下的本底。A plutonium multi-channel γ-ray spectrum at 92 to 112 keV contains 8 γ-ray lines and 29 X-ray lines which are decayed from 238Pu,239Pu,240Pu,241Pu and 241Am. CMGA can provide isotopes abundances of a sample by analyzing its spectrum in this region. After unfolding γ-ray spectra of two samples （each sample has been measured 6 times）, the value of 240Pu/239Pu given by CMGA2.0 normalized to that measured with mass spectrum method is 1.010±0.008 for sample 1 and 0.995±0.011 for sample 2, respectively. Precision of the results was comparatable with that from MGA and FRAM. Comparing the different fitting results from CMGA2.0 with different methods for describing the background shape, it is found that bilinear step background method can accurately describe the background shape in the multi-peak region.

关 键 词：Pu同位素丰度 多通道γ能谱 非破坏分析 本底 

分 类 号：O657.62[理学—分析化学] O571.23[理学—化学]