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出 处:《岩矿测试》2010年第6期655-658,共4页Rock and Mineral Analysis
基 金:国土资源地质大调查项目资助(199920190114;20020190118)
摘 要:提取、纯化海相沉积颗粒表面"诱导吸附"的36Cl(和Cl),制成加速器质谱(AMS)测定放射性比度I(36Cl/Cl)所需的标准样品,即高纯度AgCl;定量计算出沉积颗粒沉积封闭时的放射性比度I0(36Cl/Cl),依据放射性衰败定律I=I0e-λt计算得到沉积年龄t。研究结果表明:年轻的海相沉积物沉积封闭时的36Cl放射性比度I0与地理纬度之间存在一定比例关系,采取具有代表性、无污染的太平洋表面海水(4°18′N,161°09′E),经AMS测出的36Cl放射性比度IL为99.34±10.30,再利用36Cl产率与纬度的关系图,得出"放射性比度-产率"的比例常数μ为23.65238。测定了两个海底沉积物和一个海底锰结核的放射性比度I,计算得到的沉积年龄分别为83.2×104a、74.0×104a、17.6×104a。文章提出的I0定值计算方法具有科学依据,可操作性强,为揭示海洋沉积地层相关关系和沉积年龄精确测定提供技术支撑。Accelerate mass spectrometry(AMS) has been used to the measurement of specific activity I(^36Cl/Cl) of high purity AgCl made of "inducing-adsorbed" ^36Cl(and Cl) collected and purified from the surface of young marine sediments.Sediment age(t) was calculated from closed specific activity I0(^36Cl/Cl) of sediment grain based on the radioactive decay law I=I0e-λt.The study shows that the specific activity I0 of closed ^36Cl in earlier marine sediment has linear relationship with latitude.^36Cl specific activity IL from typical and uncontaminated seawater of the Pacific Ocean(4°18′N,161°09′E) surface was measured by AMS and the result was 99.34±10.30.And taking account of latitude factor,the proportionality constant of specific activity-yield(μ) was obtained as 23.65238.36Cl specific activity of two sediments grains and a manganese nodule from seabed has measured and the ages of sedimentation for the samples are 83.2×10^4 a,74.0×10^4 a and 17.6×10^4 a,respectively.The calculation method of I0 is of scientific foundation and accessibility and it can provide the exact sedimentation ages and explain the correlation of marine sediment layers.
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