Middle Stratospheric Polar Vortex Ozone Budget during the Warming Arctic Winter, 2002-2003  

作　　者：刘毅 刘传熙 铁学熙 高守亭 

机构地区：[1]Key Laboratory of Middle Atmosphere and Global Environment Observation,Institute of Atmospheric Physics,Chinese Academy of Sciences,Beijing 100029 [2]Graduate University of Chinese Academy of Sciences,Beijing 100049 [3]National Center for Atmospheric Research,Boulder,Colorado,USA [4]Laboratory of Cloud Precipitation Physicsand Severe Storms,Institute of Atmospheric Physics,Chinese Academy of Sciences,Beijing 100029

出　　处：《Advances in Atmospheric Sciences》2011年第5期985-996,共12页大气科学进展（英文版）

基　　金：funded by the National Natural Science Foundation of China under Grant No.40633015;the National Basic Research Program of China under Grant No.2010CB428604;the Dragon 2 Programme (ID:5311);The National Center for Atmospheric Research is sponsored by the National Science Foundation of the USA

摘　　要：The ozone budget inside the middle stratospheric polar vortex （24-36 km） during the 2002-2003 Arctic winter is studied by analyzing Michelson Interferometer for Passive Atmospheric Sounding （MIPAS） satellite data.A comprehensive global chemical transport model （Model for Ozone and Related Chemical Tracers,MOZART-3） is used to analyze the observed variation in polar vortex ozone during the stratospheric sudden warming （SSW） events.Both MIPAS measurement and MOZART-3 calculation show that a pronounced increase （26-28 DU） in the polar vortex ozone due to the SSW events.Due to the weakening of the polar vortex,the exchange of ozone mass across the edge of the polar vortex increases substantially and amounts to about 3.0 × 10 7 kg according to MOZART-3 calculation.The enhanced downward transport offsets about 80% of polar vortex ozone mass increase by horizontal transport.A ＂passive ozone＂ experiment shows that only ～55% of the vertical ozone mass flux in February and March can be attributed to the variation in vertical transport.It is also shown that the enhanced downward ozone above ～32 km should be attributed to the springtime photochemical ozone production.Due to the increase of air temperature,the NO x reaction rate increases by 40%-80% during the SSW events.As a result,NO x catalytic cycle causes another 44% decrease in polar vortex ozone compared to the net ozone changes due to dynamical transport.It is also shown that the largest change in polar vortex ozone is due to horizontal advection by planetary waves in January 2003.The ozone budget inside the middle stratospheric polar vortex （24-36 km） during the 2002-2003 Arctic winter is studied by analyzing Michelson Interferometer for Passive Atmospheric Sounding （MIPAS） satellite data.A comprehensive global chemical transport model （Model for Ozone and Related Chemical Tracers,MOZART-3） is used to analyze the observed variation in polar vortex ozone during the stratospheric sudden warming （SSW） events.Both MIPAS measurement and MOZART-3 calculation show that a pronounced increase （26-28 DU） in the polar vortex ozone due to the SSW events.Due to the weakening of the polar vortex,the exchange of ozone mass across the edge of the polar vortex increases substantially and amounts to about 3.0 × 10 7 kg according to MOZART-3 calculation.The enhanced downward transport offsets about 80% of polar vortex ozone mass increase by horizontal transport.A ＂passive ozone＂ experiment shows that only ～55% of the vertical ozone mass flux in February and March can be attributed to the variation in vertical transport.It is also shown that the enhanced downward ozone above ～32 km should be attributed to the springtime photochemical ozone production.Due to the increase of air temperature,the NO x reaction rate increases by 40%-80% during the SSW events.As a result,NO x catalytic cycle causes another 44% decrease in polar vortex ozone compared to the net ozone changes due to dynamical transport.It is also shown that the largest change in polar vortex ozone is due to horizontal advection by planetary waves in January 2003.

关 键 词：stratospheric sudden warming planetary wave MIPAS MOZART-3 model ozone depletion 

分 类 号：P467[天文地球—大气科学及气象学]