大气颗粒物中^(129)I的加速器质谱测量  

Measurement of ^(129)I Concentration in Air Particle Samples by AMS

作　　者：谢林波[1,2] 李奇[3] 王世联[3] 何明[2] 董克君[2] 拓飞[4] 武绍勇[2] 刘广山[1] 姜山[2] 

机构地区：[1]厦门大学环境与生态学院,福建厦门361102 [2]中国原子能科学研究院核物理研究所,北京102413 [3]禁核试北京国家数据中心和北京放射性核素实验室,北京100085 [4]中国疾病预防控制中心辐射防护与核安全医学所,北京102206

出　　处：《原子能科学技术》2014年第9期1675-1680,共6页Atomic Energy Science and Technology

基　　金：国家自然科学基金资助项目(11075221)

摘　　要：建立了通过制备大气颗粒物中碘样品并采用加速器质谱(AMS)测量颗粒物样品中129I浓度的方法。采用此方法对日本福岛核电站泄漏事故期间北京大气颗粒物样品进行了129I测量,以此探讨129I在环境监测中的作用。北京地区大气颗粒物129I的测量结果显示,2011年3月26日的大气颗粒物中129I浓度已高于正常本底值的数倍,据推测这部分129I来源于福岛核电站泄漏事故。129I是重要的核裂变产物,其来源具有特殊性,较长的半衰期使其在核反应堆中长期积累,核泄漏早期存在区域环境高浓度129I现象,所以129I-AMS测量在辐射安全及应急监测方面具有潜在优势。A method to measure the 129 I concentration in air particle samples using accel-erator mass spectrometry （AMS） was developed ,together with the preparation of AgI target of air particle .At the same time ,for the radiation monitoring use ,the measure-ment of 129I during the accident of Fukushima Nuclear Power Plant （FNPP） with the AMS facility at the China Institute of Atomic Energy （CIAE） was discussed . The results show that early on March 26 ,2011 ,129 I derived from FNPP accident had arrived and the 129 I concentration in air particle increased greatly relative to the background＆amp;nbsp;value .Due to the long half life of 129 I and its accumulation in the NPP ,the event of regional high 129 I concentration occurs in the early stage of the nuclear leakage ,conse-quently ,and the 129 I-AMS measurement has great potential to be applied for radiation safety and emergency monitoring .

关 键 词：加速器质谱 大气颗粒物 ^129I 福岛核电站事故 环境监测 

分 类 号：TL817.4[核科学技术—核技术及应用]