Distribution and transportation of mercury from glacier to lake in the Qiangyong Glacier Basin, southern Tibetan Plateau, China  

作　　者：Shiwei Sun 

机构地区：[1]State Key Laboratory of Cryospheric Sciences, Cold and Arid Regions Environmental and Engineering Research Institute, Chinese Academy of Sdences (CAS), Lanzhou 730000, China [2]Key Laboratory of Tibetan Environment Changes and Land Surface Processes, Institute of Tibetan Plateau Research, CAS, Beijing 100101, China [3]CAS Center for Excellence in Tibetan Plateau Earth Sciences, Beijing 100101, China [4]Laboratory of Green Chemistry, Lappeenranta University of Technology, Sammonkatu 12, F1-50130 Mikkeli, Finland [5]University of Chinese Academy of Sciences, Beijing 100049, China [6]Himalayan Environment Research Institute (HERI), Bauddha-6, Kathmandu, Nepal

出　　处：《Journal of Environmental Sciences》2016年第6期213-223,共11页环境科学学报（英文版）

基　　金：supported by the National Natural Science Foundation of China (Nos. 41121001, 41225002, 41571073);the Strategic Priority Research Program (B) of the Chinese Academy of Sciences (No. XDB03030504)

摘　　要：The Tibetan Plateau is home to the largest aggregate of glaciers outside the Polar Regions and is a source of fresh water to 1.4 billion people. Yet little is known about the transportation and cycling of Hg in high-elevation glacier basins on Tibetan Plateau. In this study, surface snow,glacier melting stream water and lake water samples were collected from the Qiangyong Glacier Basin. The spatiotemporal distribution and transportation of Hg from glacier to lake were investigated. Significant diurnal variations of dissolved Hg（DHg） concentrations were observed in the river water, with low concentrations in the morning（8：00 am–14：00 pm） and high concentrations in the afternoon（16：00 pm–20：00 pm）. The DHg concentrations were exponentially correlated with runoff, which indicated that runoff was the dominant factor affecting DHg concentrations in the river water. Moreover, significant decreases of Hg were observed during transportation from glacier to lake. DHg adsorption onto particulates followed by the sedimentation of particulate-bound Hg（PHg） could be possible as an important Hg removal mechanism during the transportation process. Significant decreases in Hg concentrations were observed downstream of Xiao Qiangyong Lake, which indicated that the high-elevation lake system could significantly affect the distribution and transportation of Hg in the Qiangyong Glacier Basin.The Tibetan Plateau is home to the largest aggregate of glaciers outside the Polar Regions and is a source of fresh water to 1.4 billion people. Yet little is known about the transportation and cycling of Hg in high-elevation glacier basins on Tibetan Plateau. In this study, surface snow,glacier melting stream water and lake water samples were collected from the Qiangyong Glacier Basin. The spatiotemporal distribution and transportation of Hg from glacier to lake were investigated. Significant diurnal variations of dissolved Hg（DHg） concentrations were observed in the river water, with low concentrations in the morning（8：00 am–14：00 pm） and high concentrations in the afternoon（16：00 pm–20：00 pm）. The DHg concentrations were exponentially correlated with runoff, which indicated that runoff was the dominant factor affecting DHg concentrations in the river water. Moreover, significant decreases of Hg were observed during transportation from glacier to lake. DHg adsorption onto particulates followed by the sedimentation of particulate-bound Hg（PHg） could be possible as an important Hg removal mechanism during the transportation process. Significant decreases in Hg concentrations were observed downstream of Xiao Qiangyong Lake, which indicated that the high-elevation lake system could significantly affect the distribution and transportation of Hg in the Qiangyong Glacier Basin.

关 键 词：Mercury Glacier River water Lake water Transportation Tibetan Plateau 

分 类 号：X51[环境科学与工程—环境工程] TM406[电气工程—电器]