机构地区:[1]National Laboratory for Superconductivity, Beijing National Laboratory for Condensed Matter Physics, Institute of Physics,Chinese Academy of Sciences, Beijing 100190, China [2]Brookhaven National Laboratory, Condensed Matter Physics and Materials Science Department, New York, NY 11973, USA [3]Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing 100190, China [4]Collaborative Innovation Center of Quantum Matter,Beijing 100871, China
出 处:《Science Bulletin》2016年第13期1037-1043,共7页科学通报(英文版)
基 金:XJZ thanks financial support from the National Natural Science foundation of China (11190022,11334010 and 11534007);the National Basic Research Program of China (2015CB921000);the Strategic Priority Research Program (B) of Chinese Academy of Sciences (XDB07020300)
摘 要:We report a successful tuning of the hole doping level over a wide range in high temperature superconductor Bi2Sr2CaCu2O8+δ (Bi2212) through successive in situ potassium (K) deposition. By taking high resolution angleresolved photoemission measurements on the Fermi surface and band structure of an overdoped Bi2212 (To = 76 K) at different stages of K deposition, we found that the area of the hole-like Fermi surface around the Brillouin zone corner (n,n) shrinks with increasing K deposition. This indicates a continuous hole concentration change from initial - 0.26 to eventual 0.09 after extensive K deposition, a net doping level change of 0.17 that makes it possible to bring Bi2212 from being originally overdoped, to optimally-doped, and even- tually becoming heavily underdoped. The electronic behaviors with K deposition are consistent with those of Bi2212 samples with different hole doping levels. These results demonstrate that K deposition is an effective way of in situ controlling the hole concentration in Bi2212. This work opens a good way of studying the doping evolution of electronic structure and establishing the electronic phase diagram in Bi2212 that can be extended to other cuprate superconductors.We report a successful tuning of the hole doping level over a wide range in high temperature superconductor Bi_2Sr_2CaCu_2O_(8+δ)(Bi2212) through successive in situ potassium(K) deposition. By taking high resolution angleresolved photoemission measurements on the Fermi surface and band structure of an overdoped Bi2212(T_c= 76 K) at different stages of K deposition, we found that the area of the hole-like Fermi surface around the Brillouin zone corner(p,p) shrinks with increasing K deposition. This indicates a continuous hole concentration change from initial 0.26 to eventual 0.09 after extensive K deposition, a net doping level change of 0.17 that makes it possible to bring Bi2212 from being originally overdoped, to optimally-doped, and eventually becoming heavily underdoped. The electronic behaviors with K deposition are consistent with those of Bi2212 samples with different hole doping levels. These results demonstrate that K deposition is an effective way of in situ controlling the hole concentration in Bi2212. This work opens a good way of studying the doping evolution of electronic structure and establishing the electronic phase diagram in Bi2212 that can be extended to other cuprate superconductors.
关 键 词:Bi2212 - Superconductor- K-deposition -Photoemission Fermi surface
分 类 号:TM26[一般工业技术—材料科学与工程]
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