Screening the emission sources of volatile organic compounds （VOCs） in China by multi-effects evaluation  

作　　者：He NIU Ziwei MO Min SHAO Sihua LU ShaodongXIE 

机构地区：[1]State Joint Key Laboratory of Environmental Simulation and Pollution Control, College of Environmental Science and Engineering, Peking University, Beijing 100871, China

出　　处：《Frontiers of Environmental Science & Engineering》2016年第5期25-35,共11页环境科学与工程前沿（英文）

基　　金：This study was funded by the Natural Science Foundation for Outstanding Young Scholars （Grant No. 41125018） and Natural Science Foundation Key Project （Grant No. 41330635）. The fimding source was involved in the data collection of this paper.

摘　　要：Volatile organic compounds （VOCs） play important roles in the atmosphere via three main pathways： photochemical ozone formation, secondary organic aerosol production, and direct toxicity to humans. Fewstudies have integrated these effect, s to prioritize control measures for VOC.s sources. In this study,we developed a multi-effects evaluation methodology based on updated emission inventories and source profiles, by combining the ozone formation potential （OFP）, secondary organic aerosol potential （SOAP）, and VOC toxicity data. We derived species-specific emission inventories for 152 sources. The OFPs, SOAPs, and toxicity of each source were estimated, the contribution and sharing of source to each of these adverse effects were calculated. Weightings were given to the three adverse effects by expert scoring, and then the integrated effect was determined. Taking 2012 as the base year,solvent use and industrial process were found to be the most important anthropogenic sources, accounting for 24.2% and 23.1% of the integrated effect, respectively, followed by biomass burning, transportation, and fossil fuel combustion, each had a similar contribution ranging from 16.7% to 18.6%. The top five industrial sources, including plastic products, rubber products, chemical fiberproducts, the chemical industry, and oil refining, accounted for nearly 70.0% of industrial emissions. Beijing, Chongqing, Shanghai, Jiangsu, and Guangdong were the five provinces contributing the largest integrated effects. For the VOC species from emissions showed the largest contributions were styrene, toluene, ethylene, benzene, and m/p-xylene.Volatile organic compounds （VOCs） play important roles in the atmosphere via three main pathways： photochemical ozone formation, secondary organic aerosol production, and direct toxicity to humans. Fewstudies have integrated these effect, s to prioritize control measures for VOC.s sources. In this study,we developed a multi-effects evaluation methodology based on updated emission inventories and source profiles, by combining the ozone formation potential （OFP）, secondary organic aerosol potential （SOAP）, and VOC toxicity data. We derived species-specific emission inventories for 152 sources. The OFPs, SOAPs, and toxicity of each source were estimated, the contribution and sharing of source to each of these adverse effects were calculated. Weightings were given to the three adverse effects by expert scoring, and then the integrated effect was determined. Taking 2012 as the base year,solvent use and industrial process were found to be the most important anthropogenic sources, accounting for 24.2% and 23.1% of the integrated effect, respectively, followed by biomass burning, transportation, and fossil fuel combustion, each had a similar contribution ranging from 16.7% to 18.6%. The top five industrial sources, including plastic products, rubber products, chemical fiberproducts, the chemical industry, and oil refining, accounted for nearly 70.0% of industrial emissions. Beijing, Chongqing, Shanghai, Jiangsu, and Guangdong were the five provinces contributing the largest integrated effects. For the VOC species from emissions showed the largest contributions were styrene, toluene, ethylene, benzene, and m/p-xylene.

关 键 词：Ozone formation Secondary organic aerosol Multi-effects evaluation VOC abatement strategy 

分 类 号：X51[环境科学与工程—环境工程] X701