稀土氯化物喷雾热解装置雾化效果的物理模拟  

Physical Simulation of Atomization Effect of Rare-Earth Chloride Spray Pyrolysis Device

作　　者：刘燕[1] 李小龙[1] 张宸[1] 张子木[1] LIU Yan;LI Xiao-long;ZHANG Chen;ZHANG Zi-mu(Key Laboratory for Ecological Metallurgy of Multimetallic Mineral(Ministry of Education),Northeastern University,Shenyang 110819,China)

机构地区：[1]东北大学多金属共生矿生态化冶金教育部重点实验室,辽宁沈阳110819

出　　处：《东北大学学报（自然科学版）》2019年第2期218-223,共6页Journal of Northeastern University(Natural Science)

基　　金：国家自然科学基金-云南联合重点基金资助项目(U1402271);国家重点研发计划项目(2017YFC0210403)

摘　　要：稀土氯化物雾化热解是稀土氧化物制备新工艺,但目前喷雾热解装备雾化效果差,雾化后液滴粒径分布不均匀.本文自行设计了文丘里管喷雾热解反应器,将粒子图像测速技术与MATLAB图像处理技术相结合,研究了气体流量、文丘里管和引流管几何尺寸等因素对雾化效果的影响.结果表明:文丘里管扩散段中较强的回流作用会加剧气液相间的混合碰撞,进一步破碎液滴;而过多的液相携带量容易导致雾滴密度变大,增大了液滴在运动过程中的碰撞几率,致使雾滴尺寸变大.文丘里管反应器适宜的几何尺寸和操作条件为:内径100 mm,喉口内径10 mm,引流管内径5 mm,气相流量20.5 m3/h.Spray pyrolysis rare-earth chloride is a new process to produce rare-earth oxides,but there are some shortages at present such as the poor atomization effect of spray pyrolysis equipment and the non-uniform distribution of the droplet size after atomization.A Venturi tube spray pyrolysis reactor was designed and particle image velocimetry technology combined with MATLAB image processing technology was used to analyze the effects of gas flow rate,the size of Venturi tube and drainage tube on the atomization.The results show that the strong back-flow in the diffuser of Venturi tube can intensify the collision of gas-liquid phases and crush more drops,while the excessive amount of liquid phase in the Venturi tube increases the droplet density and collision probability of droplet in motion,leading to larger droplet size.The suitable geometric size for Venturi tube reactor are 100 mm-inner diameter,10 mm-throat diameter,5 mm-inner diameter of drainage tube and the gas flow rate of 20.5 m^3/h.

关 键 词：喷雾热解 稀土氧化物 文丘里射流反应器 雾化效果 图像处理 

分 类 号：TF845[冶金工程—有色金属冶金]