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作 者:Yazhao Liu Zhi hao Li Guangwen Chu Lei Shao Yong Luo Jianfeng Chen
机构地区:[1]Research Center of the Ministry of Education for High Gravity Engineering and Technology,Beijing 100029,China [2]State Key Laboratory of Organic-Inorganic Composites,Beijing University of Chemical Technology,Beijing 100029,China
出 处:《Chinese Journal of Chemical Engineering》2020年第10期2507-2512,共6页中国化学工程学报(英文版)
基 金:supported by the National Natural Science Foundation of China(Nos.21676009 and 21725601)。
摘 要:A rotating packed bed(RPB) reactor has substantially potential for the process intensification of heterogeneous catalytic reactions. However, the scarce knowledge of the liquid–solid mass transfer in the RPB reactor is a barrier for its design and scale-up. In this work, the liquid–solid mass transfer in a RPB reactor installed with structured foam packing was experimentally studied using copper dissolution by potassium dichromate. Effects of rotational speed, liquid and gas volumetric flow rate on the liquid–solid mass transfer coefficient(kLS) have been investigated. The correlation for predicting kLSwas proposed, and the deviation between the experimental and predicted values was within±12%. The liquid–solid volumetric mass transfer coefficient(kLSaLS) ranged from 0.04–0.14 1^-1, which was approximately 5 times larger than that in the packed bed reactor. This work lays the foundation for modeling of the RPB reactor packed with structured foam packing for heterogeneous catalytic reaction.
关 键 词:Rotating packed bed Liquid–solid mass transfer Structured foam packing Process intensification
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