二维材料用于电催化析氢的研究进展  

Recent Advances of Two-dimensional Materials for Electrocatalytic Hydrogen Evolution

作　　者：史江维 孟楠楠[2] 郭亚梅 于一夫[2] 张兵[1] SHI Jiangwei;MENG Nannan;GUO Yamei;YU Yifu;ZHANG Bin(Department of Industrial Catalysis,School of Chemical Engineering and Technology,School of Science;Institute of Molecular Plus,Tianjin University,Tianjin 300072,China)

机构地区：[1]天津大学化工学院工业催化系,理学院 [2]天津大学分子+研究院,天津300072

出　　处：《高等学校化学学报》2021年第2期492-503,共12页Chemical Journal of Chinese Universities

基　　金：国家自然科学基金(批准号:22071173,21701122);天津市自然科学基金(批准号:17JCJQJC44700)资助.

摘　　要：电催化水分解因其丰富的原料来源和环境友好被认为是一种有前途的制氢技术.开发用于电催化析氢反应的高效电催化剂是迫切需要的.随着石墨烯的兴起,二维(2D)材料因其独特的物理、化学和电子特性,已逐渐成为水电解的潜在候选材料.本文介绍了二维材料用于电化学水分解产生氢气的最新进展,概括了二维材料的合成方法,总结了改善二维材料电化学析氢性能的策略,讨论了该领域面临的挑战和未来的发展机遇.Electrocatalytic water splitting is considered as a promising technique to produce hydrogen due to its abundant source and environmental friendliness.The development of efficient electrocatalysts for electrocatalytic hydrogen evolution reaction(HER)is highly desirable.With the rise of graphene,two-dimensional(2D)materials have become a potential candidate in water electrolysis due to their unique physical,chemical,and electronic properties.Herein,this review sumarized the recent advances of 2D materials for electrochemical water splitting to produce hydrogen.Firstly,synthesis methods for 2D materials were introduced.Subsequently,strategies to improve the HER performance of 2D materials were summarized.Finally,some challenges and future opportunities in this field were summarized and proposed.

关 键 词：电催化 析氢反应 纳米材料 二维材料 水分解 

分 类 号：O643[理学—物理化学]