New Horizon in stabilization of single atoms on metal-oxide supports for CO_(2) reduction  

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作  者:Muhammad Abbas Muhammad Aurang Zeb Gul Sial 

机构地区:[1]Department of Chemistry and Biochemistry,The University of Texas at Dallas,800 West Campbell Road,Richardson,TX,75080,USA [2]Multi-scale Porous Materials Centre,Institute of Advanced Interdisciplinary Studies,School of Chemistry and Chemical Engineering,Chongqing University,Chonging,400044,PR China

出  处:《Nano Materials Science》2021年第4期368-389,共22页纳米材料科学(英文版)

基  金:This work was supported by China Postdoctoral Science Foundation under project number 2019M663054.

摘  要:Elecrochemical CO_(2) reduction is a promising route to convert CO_(2) into the value added chemicals,and to control the increasing accumulation of 002 in the atmosphere.The CO_(2) molecule is stable and chemically inert,so a highly efficient electrocatalyst is required for CO_(2) reduction.The single atoms with metal oxdde support is a new fronder in CO_(2) reduction.The supported single atoms contain disperse isolated atoms with an appropriate support maxcimize the atom efficiency of metals for boosting the catalytc perfomance.In this review,we had discussed state-of-the-art research on the synthestis of single atoms supported on the metal oxdde for boosting catalytic activity for CO_(2) reduction and special emphasis is placed on the influence of single atoms supported on metal oxdde on the CO_(2) reduction.Futhermore,we had discussed the challenges,and opportunities for paving the development of single atoms with metal support and their application in ecrocatalytic CO_(2) reduction.

关 键 词:Single atoms Metal-oxides support CO_(2)reduction 

分 类 号:O643.36[理学—物理化学] X701[理学—化学]

 

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