A strategic review on processing routes towards scalable fabrication of perovskite solar cells  

作　　者：Yingzhuang Ma Qing Zhao 

机构地区：[1]Wenzheng College of Soochow University,Suzhou 215104,Jiangsu,China [2]State Key Lab for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics,School of Physics,Peking University,Beijing 100871,China [3]Peking University Yangtze Delta Institute of Optoelectronics,Nantong 226010,Jiangsu,China

出　　处：《Journal of Energy Chemistry》2022年第1期538-560,I0014,共24页能源化学（英文版）

基　　金：supported by the National Key Research and Development Program of China(Nos.2019YFA0707003 and 2019YFE0114100);the National Natural Science Foundation of China(NSFC 51872007);Beijing Municipal Natural Science Foundation(No.7202094).

摘　　要：Perovskite solar cells have reached a power-conversion efficiency(PCE) of 25.6%,showing great potential with reliable moisture and heat stability.Most results are achieved on small-area devices,using conventional thin-film processing technologies like spin-coating method.However,such approaches may not be upscaled for large-area substrates.Thus,strategies and materials need to be developed for manufacturing processing routes to realize future commercial photovoltaic fabrications.Notable results have been achieved on large-area perovskite solar cells.In this review,similarities and differences of large-area perovskite fabrication mechanisms between the various pathways are investigated,especially on the parameters affecting the nucleation and crystal growth kinetics.Moreover,the methods for large-area transporting layers and electrodes are discussed,and some key issues from cells to modules.Challenges and opportunities are proposed to pave the way of high-efficiency perovskite solar modules.

关 键 词：PEROVSKITE Solar cell LARGE-AREA COMMERCIALIZATION Scalable fabrication 

分 类 号：TB34[一般工业技术—材料科学与工程] TM914.4[电气工程—电力电子与电力传动]