CO_(2)光热催化还原研究进展  

Recent advances in photothermal catalysis of CO_(2) reduction

作　　者：闫帅 杨海平[1] 陈应泉[1] 王贤华[1] 曾阔[1] 陈汉平[1] YAN Shuai;YANG Haiping;CHEN Yingquan;WANG Xianhua;ZENG Kuo;CHEN Hanping(State Key Laboratory of Coal Combustion,Huazhong University of Science and Technology,Wuhan 430074,Hubei,China)

机构地区：[1]华中科技大学煤燃烧国家重点实验室,湖北武汉430074

出　　处：《化工学报》2022年第10期4298-4310,共13页CIESC Journal

基　　金：国家杰出青年科学基金项目(52125601)。

摘　　要：CO_(2)光热催化转化是一种新型的CO_(2)利用技术,该过程绿色、经济且无须额外能量输入,是当下的热门研究领域之一。本文主要总结了CO_(2)光热催化转化领域的最新研究进展,介绍了基于光热转化的光热催化剂设计方法,同时从光热催化机理出发解析了CO_(2)还原反应的光热催化剂构建策略,并揭示了CO_(2)还原反应中的光热协同耦合机制,为光热催化剂的设计以及CO_(2)的高效转化和利用提供参考。Photothermal catalytic conversion of CO_(2) is a new type of CO_(2) utilization technology.The process is green,economical,and requires no additional energy input.It is one of the current hot research fields.This paper introduced recent advances in photothermal catalytic conversion of CO_(2) and summarized design methods for photothermal catalysts based on photo-to-thermal conversion.In addition,fabrication strategies were also investigated in the perspective of photothermal catalytic mechanism and the synergy between photo-and thermo effects was also discussed.This work aims to promote the understanding of photothermal synergy for CO_(2) reduction reaction and provides reference for the design of photothermal catalysts and CO_(2) valorization.

关 键 词：CO_(2)利用 光热催化 光热转化 催化剂设计 

分 类 号：TQ032[化学工程]