Features of ^(90)Sr behavior in Crimean lakes with different salinity of their water environment  

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作  者:N.Yu.Mirzoeva S.I.Arkhipova V.Yu.Proskurnin O.N.Miroshnichenko I.N.Moseichenko 

机构地区:[1]A.O.Kovalevsky Institute of Biology of the Southern Seas of RAS,Sevastopol,Russian Federation

出  处:《Acta Geochimica》2023年第1期89-102,共14页地球化学学报(英文)

基  金:Scientific research on salt and brackish water lakes was supported by the Russian Science Foundation,with grant No.18-16-00001;Development of biological and geochemical foundations for the development of aquaculture in hypersaline lakes and lagoons of Crimea,2021-2022;Comparative studies on the Black Sea were carried out within the framework of the State Assignment for the IBSS,Molismological and biogeochemical foundations of the homeostasis of marine ecosystems,with State registration number of the state assignment 121031500515-8。

摘  要:The comparative study of technogenic ^(90)Sr behavior features in Crimea lakes’ ecosystems with different levels of salinity was carried out in 2016-2021.Two sources of ^(90)Sr input were identified for all the studied lakes:the primary source concerned with atmospheric fallout immediately after the Chernobyl NPP accident and the secondary long-term input of this radionuclide by waterway.The half-life of the ^(90)Sr concentration in the water of the hypers aline Lake Sasyk-Sivash was estimated to vary from 0.8 to 1.1 years after the closure of the North Crimean Canal(NCC).Biogeochemical processes in the lake under the absence of the secondary source of the radionuclide input were shown to decrease in the ^(90)Sr residence time in the water column by 131 times.For brackish water bodies,a significant factor influencing the radionuclide concentration in ecosystems of lakes was the pH of their water,while for hypers aline lakes the level of water salinity was the main factor determining ^(90)Sr behavior.The concentration of ^(90)Sr in bottom sediments of studied lakes depended mainly on this radionuclide concentration in a water environment.Calculated ^(90)Sr distribution factors(Kd) for studied lakes’ bottom sediments varied in a range of n·10^(0)÷n·10^(2) for hypersaline lakes and of n·10^(1)÷n·10^(2) for lakes with brackish waters.Due to the closure of the NCC,the ^(90)Sr redistribution took place in lake ecosystems only under the geochemical processes within the water bodies themselves.The results obtained in this work are of particular importance as a starting point or a basis for further radioecological studies of the Crimean inland waters after the reopening of the NCC and the Dnieper waters re-entering the territory of Crimea in 2022after the 8 years of their absence.

关 键 词:^(90)Sr Salt lakes Water Bottom sediments Chernobyl NPP accident CRIMEA 

分 类 号:P343.3[天文地球—水文科学] P512.2[天文地球—地球物理学]

 

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