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作 者:蔡斌[1] 程昊淼 亓浩雲 李奥哲 康天放[1] CAI Bin;CHENG Hao-miao;QI Hao-yun;LI Ao-zhe;KANG Tian-fang(Key Laboratory of Beijing on Regional Air Pollution Control,Department of Environment and Life Sciences,Beijing University of Technology,Beijing 100124,China;College of Architecture and Urban Planning,Department of Architecture,Civil and Transportation Engineering,Beijing University of Technology,Beijing 100124,China)
机构地区:[1]北京工业大学环境与生命学部,区域大气复合污染防治北京市重点实验室,北京100124 [2]北京工业大学城市建设学部,建筑与城市规划学院,北京100124
出 处:《中国环境科学》2023年第6期2734-2743,共10页China Environmental Science
基 金:国家自然科学基金资助项目(52170174)。
摘 要:以京津冀地区BVOCs排放清单为基础,采用WRF-CMAQ模型模拟与情景分析相结合的方式研究了2018年7月京津冀地区BVOCs排放对O_(3)和PM_(2.5)浓度贡献,解析了北京、邯郸、承德、保定等典型城市不同植被类型BVOCs排放对O_(3)和SOA浓度的影响水平,并应用O_(3)和SOA生成潜势核算结果对模拟结果进行验证.结果显示,BVOCs排放对北京、邯郸、承德、保定O_(3)生成贡献率分别为30.19%、24.77%、35.56%、26.73%,对SOA生成贡献率为2.55%、3.32%、4.17%、3.59%;北京、承德的乔木与果园BVOCs排放对O_(3)和SOA浓度贡献最大,邯郸、保定的草地与庄稼BVOCs排放对O_(3)和SOA浓度贡献最大;数值模拟结果与O_(3)、SOA生成潜势表征的潜在影响基本符合.Based on the BVOCs emission inventory,WRF-CMAQ model was used with scenario analysis to investigate the effects of BVOCs emissions on O_(3)and PM_(2.5) in the Beijing-Tianjin-Hebei region in July 2018.The effects of BVOCs emissions from different vegetation types on O_(3)and SOA concentrations in Beijing,Handan,Chengde,Baoding and other cities were quantitatively analyzed,which was verified with the O_(3)and SOA formation potential method.As the results showed,the contributions of BVOCs emission to O_(3)in Beijing,Handan,Chengde and Baoding were 30.19%,24.77%,35.56%and 26.73%,respectively,and the contributions to SOA were 2.55%,3.32%,4.17%and 3.59%,respectively.Trees and orchards showed the greatest influences on O_(3)and SOA in Beijing and Chengde,while grassland and crops showed the greatest contributions in Handan and Baoding.Additionally,the results of numerical simulation and of potential generation method showed relatively consistent results.
关 键 词:植被功能类型 BVOCs O_(3)和SOA WRF-CMAQ 生成潜势
分 类 号:X513[环境科学与工程—环境工程]
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