Advances in solid Mg-ion electrolytes for solid-state Mg batteries  

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作  者:Yuepeng Pang Yu Zhu Fang Fang Dalin Sun Shiyou Zheng 

机构地区:[1]School of Materials and Chemistry,University of Shanghai for Science and Technology,Shanghai 200093,China [2]Department of Materials Science,Fudan University,Shanghai 200433,China

出  处:《Journal of Materials Science & Technology》2023年第30期136-149,共14页材料科学技术(英文版)

基  金:The authors gratefully acknowledge the support of the National Natural Science Foundation of China(Nos.51971146,51971147,52171218,and 52271222);the Shanghai Municipal Science and Technology Commission(No.21010503100);the Major Program for the Scientific Research Innovation Plan of Shanghai Education Com-mission(No.2019-01-07-00-07-E00015);the Shanghai Outstand-ing Academic Leaders Plan,the Shanghai Rising-Star Program(No.20QA1407100);the General Program of Natural Science Foun-dation of Shanghai(No.20ZR1438400).

摘  要:Rechargeable Mg batteries have attracted much attention in the past decade due to their high theoretical energy density and low production cost,in which the electrolyte is the key component that determines the overall performance.Applying solid Mg-ion electrolytes brings many benefits to rechargeable Mg bat-teries,which can improve safety under aggressive conditions and open opportunities for new electrode applications.After extensive investigations,researchers make major breakthroughs in the solid Mg-ion electrolyte field,especially in terms of Mg-ion conductivities.However,the development of solid-state Mg batteries is still at the early stage since their stable cycling has not been achieved yet.In this review,we introduce the Mg-ion conducting properties of current solid Mg-ion electrolytes,and then summarize the performances of corresponding solid-state Mg batteries.In addition,we provide a discussion on the application potentials and future directions of each type of solid Mg-ion electrolytes that are applied in solid-state Mg batteries.

关 键 词:Solid Mg-ion electrolytes Solid-state Mg batteries Phosphates BOROHYDRIDES CHALCOGENIDES Metal-organic frameworks Polymers 

分 类 号:TM912[电气工程—电力电子与电力传动]

 

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