海南岛臭氧污染时空变化及敏感性特征  

Spatial and Temporal Variations in Ozone Pollution and Sensitivity Characteristics in Hainan Island

作　　者：符传博 丹利[2] 佟金鹤[1,3] 徐文帅 FU Chuan-bo;DAN Li;TONG Jin-he;XU Wen-shuai(Hainan Institute of Meteorological Science,Haikou 570203,China;Key Laboratory of Regional Climate-Environment Research for Temperate East Asia,Institute of Atmospheric Physics,Chinese Academy of Sciences,Beijing 100029,China;Key Laboratory of South China Sea Meteorological Disaster Prevention and Mitigation of Hainan Province,Haikou 570203,China;Hainan Research Academy of Environmental Sciences,Haikou 571126,China)

机构地区：[1]海南省气象科学研究所,海口570203 [2]中国科学院大气物理研究所东亚区域气候-环境重点实验室,北京100029 [3]海南省南海气象防灾减灾重点实验室,海口570203 [4]海南省环境科学研究院,海口571126

出　　处：《环境科学》2023年第9期4799-4808,共10页Environmental Science

基　　金：国家自然科学基金项目(42065010,42141017);海南省重大科技计划项目(ZDKJ202007);海南省自然科学基金项目(422RC802,421QN0967);海南省院士创新平台科研项目(YSPTZX202143)。

摘　　要：基于环境空气质量数据、气象观测数据和卫星遥感资料,研究了2015~2020年海南岛臭氧(O_(3))污染的时空分布、变化趋势、 O_(3)生成敏感性及其与气象因子的关系.结果表明,海南岛O_(3)-8h(日最大8 h滑动平均值)表现为西部和北部偏高,中部、东部和南部偏低的分布特征,2015年O_(3)-8h浓度最高,2019年O_(3)-8h浓度超标占比最大.O_(3)-8h浓度与平均气温(P<0.1)、日照时数(P<0.01)、太阳总辐射(P<0.01)、大气压和平均风速呈正相关关系,与降雨量(P<0.05)和相对湿度呈负相关关系.卫星遥感数据显示,2015~2020年海南岛对流层NO2柱浓度(NO2-OMI)和HCHO柱浓度(HCHO-OMI)呈相反的变化趋势,2020年NO2-OMI较2015年上升了7.74%, HCHO-OMI下降了10.2%.海南岛属于NOx控制区,近6年FNR值(O_(3)生成敏感性)呈波动式地下降趋势,其趋势系数和气候倾向率分别为-0.514和-0.123 a^(-1).气象因子与海南岛FNR值有较好的相关关系.Based on ambient air quality data,meteorological observation data,and satellite remote sensing data,the temporal and spatial variations in ozone(O_(3))pollution,the sensitivity of O_(3),and its relationship with meteorological factors in Hainan Island were analyzed in this study.The results showed that the maximum daily 8⁃h moving mean(O_(3)⁃8h)in western and northern cities in Hainan Island was higher than that in the central,eastern,and southern cities.O_(3)⁃8h was the highest in 2015,and O_(3)⁃8h exceeding the standard proportion was the largest in 2019.In addition,O_(3)⁃8h was positively correlated with average temperature(P<0.1),sunshine duration(P<0.01),total solar radiation(P<0.01),atmospheric pressure,and average wind speed and was negatively correlated with precipitation(P<0.05)and relative humidity.The satellite remote sensing data showed that the tropospheric NO2 column concentration(NO2⁃OMI)and HCHO column concentration(HCHO⁃OMI)displayed opposite trends in Hainan Island from 2015 to 2020.Compared with those in 2015,NO2⁃OMI increased by 7.74%and HCHO⁃OMI decreased by 10.2%in 2020.Moreover,Hainan Island belongs to the NOx control area,and the FNR value exhibited a fluctuating downward trend in the past 6 years,with a trend coefficient and climatic trend rate of-0.514 and-0.123 a^(-1),respectively.A strong correlation was observed between meteorological factors and the FNR value of Hainan Island.

关 键 词：臭氧(O_(3)) 臭氧检测仪(OMI) 卫星监测 臭氧敏感性 海南岛 

分 类 号：X515[环境科学与工程—环境工程]