Assessing roles of geochemical reactions on CO_(2)plume,injectivity and residual trapping  

作　　者：Abdiaziz Abdullahi Maalim Hisham Ben Mahmud Mojtaba Seyyedi 

机构地区：[1]Curtin University Malaysia,CDT250,Miri,98000,Sarawak,Malaysia [2]CSIRO,GPO Box 1700,Canberra ACT,2601,Australia

出　　处：《Energy Geoscience》2021年第4期327-336,共10页能源地球科学（英文）

摘　　要：With increasing CO_(2)concentration in the atmosphere,CO_(2)geo-aequestration has become a popular technique to counter the dangers of global warming resulting from high levels of CO_(2)in the atmosphere.This paper examins sequestration parameters such as CO_(2)plume behaviour,residual gas trapping and injectivity as a means of achieving safe and successful CO_(2)storage in saline aquifers.Mineral precipitation/dissolution rates are used to establish a relationship between these parameters and geochemical reactions in saline aquifers.To achieve this,mechanistic models(6 models with different inputs,created using CMG e GEM,2016 and WINPROP,2016)are simulated using input data from literature and studying changes in fluids and formation properties as well as mineral precipitation/dissolution rates in aquifers when subjected to different conditions in the different models.The results from the models show that high CO_(2)dissolution,which creates large CO_(2)plume,leads to high mineral dissolution/precipitation as results of increased fluid-rock interactions(geochemical reactions);whereas injectivity,although enhanced by CO_(2)-water cyclic injection,does not show much increase in bottom hole pressure when mineral trapping(thus geochemical reactions)is introduced into the model.Sensitivity study on residual gas trapping shows that high residual gas saturation leads to reduced mineral precipitation/dissolution due to the reduced amount of dissolved CO_(2)in brine.Also,rapid changes in the bottom hole pressure at high residual gas saturation means that a formation that fosters high residual gas trapping,rather than CO_(2)dissolution in brine,is more likely to experience injectivity issues during the sequestration process.

关 键 词：Geochemical reactions CO_(2)plume Residual(gas)trapping INJECTIVITY Mineral precipitation Mineral dissolution 

分 类 号：P59[天文地球—地球化学]