机构地区:[1]Shenzhen Key Laboratory of Thermoelectric Materials and Department of Physics,Southern University of Science and Technology,Shenzhen 518055,China [2]Department of Electrical and Computer Engineering,National University of Singapore,Singapore 117581,Singapore [3]School of Electronic Science and Engineering,State Key Laboratory of Electronic Thin Film and Integrated Devices,University of Electronic Science and Technology of China,Chengdu 611731,China [4]Department of Materials Science and Engineering,National University of Singapore,Singapore 117575,Singapore [5]Institute of Materials Research and Engineering,Agency for Science,Technology and Research(A*STAR),Singapore 138634,Singapore [6]Guangdong-Hong Kong-Macao Joint Laboratory for Photonic-Thermal-Electrical Energy Materials and Devices,Southern University of Science and Technology,Shenzhen 518055,China
出 处:《National Science Review》2023年第9期242-251,共10页国家科学评论(英文版)
基 金:supported by the National Natural Science Foundation of China(11934007);the Guangdong-Hong Kong-Macao Joint Laboratory(2019B121205001);the Science and Technology Innovation Committee Foundation of Shenzhen(JCYJ20200109141205978);the Outstanding Talents Train-ing Fund in Shenzhen(202108);G.W.H acknowledges support by the A*STAR under its RIE2025 Manufacturing,Trade and Con-nectivity(MTC)(M22K2c0081).
摘 要:Weather-adaptive energy harvesting of omnipresent waste heat and rain droplets,though promising in the field of environmental energy sustainability,is still far from practice due to its low electrical output owing to dielectric structure irrationality and unscalability.Here we present atypical upcycling of ambient heat and raindrop energy via an all-in-one non-planar energy harvester,simultaneously increasing solar pyroelectricity and droplet-based triboelectricity by two-fold,in contrast to conventional counterparts.The delivered non-planar dielectric with high transmittance confines the solar irradiance onto a focal hotspot,offering transverse thermal field propagation towards boosted inhomogeneous polarization with a generated power density of 6.1 mW m^(−2)at 0.2 sun.Moreover,the enlarged lateral surface area of curved architecture promotes droplet spreading/separation,thus travelling the electrostatic field towards increased triboelectricity.These enhanced pyroelectric and triboelectric outputs,upgraded with advanced manufacturing,demonstrate applicability in adaptive sustainable energy harvesting on sunny,cloudy,night,and rainy days.Our findings highlight a facile yet efficient strategy,not only for weather-adaptive environmental energy recovery but also in providing key insights for spatial thermal/electrostatic field manipulation in thermoelectrics and ferroelectrics.
关 键 词:non-planar dielectrics heat manipulation PYROELECTRICS weather-adaptive energy harvesting
分 类 号:P49[天文地球—大气科学及气象学] TM619[电气工程—电力系统及自动化]
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