Meta-analysis of CO_(2) conversion,energy efficiency,and other performance data of plasma-catalysis reactors with the open access PIONEER database  

作　　者：Antoine Salden Maik Budde Carolina A.Garcia-Soto Omar Biondo Jairo Barauna Marzia Faedda Beatrice Musig ChloéFromentin Minh Nguyen-Quang Harry Philpott Golshid Hasrack Domenico Aceto Yuxiang Cai Federico Azzolina Jury Annemie Bogaerts Patrick Da Costa Richard Engeln María Elena Gálvez Timo Gans Tomas Garcia Vasco Guerra Carlos Henriques Monika Motak Maria Victoria Navarro Vasile I.Parvulescu Gerard Van Rooij Bogdan Samojeden Ana Sobota Paolo Tosi Xin Tu Olivier Guaitella 

机构地区：[1]Department of Physics,University of Trento,38100 Povo,Italy [2]Department of Applied Physics and Science Education,Eindhoven University of Technology,5600 MB Eindhoven,The Netherlands [3]Instituto de Plasmas e Fusão Nuclear,Instituto Superior Técnico,Universidade de Lisboa,1049-001 Lisboa,Portugal [4]LPP,CNRS,École Polytechnique,Sorbonne Université,UniversitéParis-Saclay,IP-Paris 91128 Palaiseau,France [5]Department of Organic Chemistry,Biochemistry and Catalysis,University of Bucharest,Bucharest,Romania [6]Research Group PLASMANT,Department of Chemistry,University of Antwerp,Universiteitsplein 1,Wilrijk B-2610,Belgium [7]DIFFER,5612AJ Eindhoven,The Netherlands [8]Instituto de Carboquímica ICB-CSIC,Zaragoza 50018,Spain [9]Faculty of Energy and Fuels,AGH University of Krakow,Krakow,Poland [10]Institut Jean le Rond d’Alembert,CNRS UMR 7190-Sorbonne Université,Saint-Cyr l’Ecole 78210,France [11]Laboratoire Catalyse et Spectrochimie(LCS),CNRS-ENSICAEN-Universitéde Caen,6 boulevard du Maréchal-Juin,14000 Caen,France [12]CQE,Centro de Química Estrutural,Instituto Superior Técnico,Universidade de Lisboa,Av.Rovisco Pais,1049-001 Lisboa,Portugal [13]School of Physical Sciences and National Centre for Plasma Science and Technology,Faculty of Science and Health,Dublin City University,Dublin,Ireland [14]ASML,De Run 6501,5504 DR Veldhoven,The Netherlands [15]Faculty of Science and Engineering,Maastricht University,6229 GS Maastricht,The Netherlands [16]CNR,Istituto per la Scienza e Tecnologia dei Plasmi(ISTP),Italy [17]Department of Electrical Engineering and Electronics,University of Liverpool,Liverpool L693GJ,UK

出　　处：《Journal of Energy Chemistry》2023年第11期318-342,I0007,共26页能源化学（英文版）

基　　金：funding from the European Union’s Horizon 2020 research and innovation programme under the Marie Sklodowska-Curie grant agreement No.813393;partially funded by the Portuguese FCT-Funda??o para a Ciência e a Tecnologia,under projects UIDB/50010/2020,UIDP/50010/2020 and PTDC/FIS-PLA/1616/2021。

摘　　要：This paper brings the comparison of performances of CO_(2)conversion by plasma and plasma-assisted catalysis based on the data collected from literature in this field,organised in an open access online database.This tool is open to all users to carry out their own analyses,but also to contributors who wish to add their data to the database in order to improve the relevance of the comparisons made,and ultimately to improve the efficiency of CO_(2)conversion by plasma-catalysis.The creation of this database and database user interface is motivated by the fact that plasma-catalysis is a fast-growing field for all CO_(2)conversion processes,be it methanation,dry reforming of methane,methanolisation,or others.As a result of this rapid increase,there is a need for a set of standard procedures to rigorously compare performances of different systems.However,this is currently not possible because the fundamental mechanisms of plasma-catalysis are still too poorly understood to define these standard procedures.Fortunately however,the accumulated data within the CO_(2)plasma-catalysis community has become large enough to warrant so-called“big data”studies more familiar in the fields of medicine and the social sciences.To enable comparisons between multiple data sets and make future research more effective,this work proposes the first database on CO_(2)conversion performances by plasma-catalysis open to the whole community.This database has been initiated in the framework of a H_(2)0_(2)0 European project and is called the“PIONEER Data Base”.The database gathers a large amount of CO_(2)conversion performance data such as conversion rate,energy efficiency,and selectivity for numerous plasma sources coupled with or without a catalyst.Each data set is associated with metadata describing the gas mixture,the plasma source,the nature of the catalyst,and the form of coupling with the plasma.Beyond the database itself,a data extraction tool with direct visualisation features or advanced filtering functionalities has been dev

关 键 词：Open-access database on plasma-catalysis experiment CO_(2) conversion PLASMA-CATALYSIS Carbon capture and utilisation(CCU) Energy efficiency Specific energy input Dielectric barrier discharge Packed bed reactor METHANATION Dry reforming of methane 

分 类 号：O643.32[理学—物理化学]