Lightnin静态混合器内气液两相混合与传质强化特性  

Enhancement of gas-liquid flow mixing and mass transfer in Lightnin static mixer

作　　者：禹言芳[1] 李毓 孟辉波 刘桓辰 YU Yanfang;LI Yu;MENG Huibo;LIU Huanchen(School of Mechanical and Power Engineering,Shenyang University of Chemical Technology,Shenyang 110142,Liaoning,China;College of New Energy,China University of Petroleum(East China),Qingdao 266580,Shandong,China)

机构地区：[1]沈阳化工大学机械与动力工程学院,辽宁沈阳110142 [2]中国石油大学(华东)新能源学院,山东青岛266580

出　　处：《化工进展》2023年第12期6180-6190,共11页Chemical Industry and Engineering Progress

基　　金：辽宁特聘教授计划(辽教函[2018]35号);国家自然科学基金(21476142);青岛市自然科学基金(23-2-1-236-zyyd-jch);辽宁省教育厅重点项目(LJKZ0429,LJKMZ20220773);辽宁省自然科学基金(2022-MS-290);中国石油大学(华东)引进人才科研基金(R20220113)。

摘　　要：采用计算流体力学(CFD)耦合群体平衡模型(PBM)研究Lightnin静态混合器(LSM)内气泡分散特性,使用不同的破碎核和聚并核函数系统研究雷诺数(Re)、气相体积分数(α_(d))和元件数量对气泡分散行为以及混合效率的影响,采用气液界面积和体积传质系数(k_(L)a)量化LSM和Kenics静态混合器(KSM)内气泡破碎性能以及传质速率,基于变异系数(CoV)和流体微元拉伸率分析LSM和KSM的分布混合性能和分散混合性能。结果表明:Luo聚并模型和Prince模型高估了LSM内气泡的聚并效率,通过Luo-Turbulent模型计算的气泡尺寸与实验数值具有很好的一致性;随着Re和α_(d)的增大,LSM内气泡的分散行为被进一步强化,在高Re的条件下增大元件数量可以显著提高气液传质效率;CoV曲线表明,LSM具有比KSM更好的分布混合性能,3个LSM元件可以保证混合程度大于95%。LSM的分散混合效率是KSM的1.06~1.16倍;基于压力波动信号时间序列,确定了LSM中流型从过渡区向非均匀区转变的临界表观速度。The bubble dispersion characteristics were investigated by computational fluid dynamics(CFD)coupled with population balance model(PBM)in the Lightnin static mixer(LSM).Different breakup and coalescence kernels were used to study the effect of Reynolds number(Re),gas volume fraction(α_(d))and the element numbers on the bubble dispersion behavior and mixing efficiency.Bubble breakup capacity and mass transfer rate were quantized via gas-liquid interfacial area and volumetric mass transfer coefficient(k_(L)a)in LSM and Kenics static mixer(KSM).The distributive mixing performance and dispersive mixing performance of LSM and KSM were analyzed based on CoV and fluid microelement stretching rate.The results showed that Luo coalescence model and Prince model overestimated the bubbles coalescence efficiency in LSM,and the bubble size calculated by the Luo-Turbulent model was Engineering Progress,2023,42(12):6180-6190.in good agreement with the experimental data.With the increase of Re andα_(d),the dispersion behavior of bubbles in LSM was further strengthened.Increasing the number of elements could significantly improve the gas-liquid mass transfer efficiency at higher Re condition.CoV curve showed that LSM had better distributive mixing performance than KSM,and three LSM elements could make the mixedness more than 95%.The dispersive mixing efficiency of LSM was 1.06 to 1.16 times that of KSM.The critical superficial velocities of flow pattern transition from pseudo-homogeneous to heterogeneous were identified based on pressure fluctuation signal time series in the LSM.

关 键 词：静态混合器 气液两相流 种群平衡公式 计算流体力学 混合 

分 类 号：TQ051.7[化学工程]