结合电子束辐照与压电压力波法空间电荷分布实时测量的空间电荷包迁移行为的研究  

Migration behavior of space charge packet researched by using electron beam irradiation and real-time space charge distribution measurement in piezo-pressure wave propagation(PWP)method

作　　者：潘佳萍 张冶文[1] 李俊 吕天华 郑飞虎[1] Pan Jia-Ping;Zhang Ye-Wen;Li Jun;LüTian-Hua;Zheng Fei-Hu(Department of Electrical Engineering,Tongji University,Shanghai 201804,China)

机构地区：[1]同济大学电子与信息工程学院,上海201804

出　　处：《物理学报》2024年第2期278-286,共9页Acta Physica Sinica

基　　金：国家自然科学基金(批准号:51877153)资助的课题。

摘　　要：空间电荷包现象是一种特殊的空间电荷现象,具体表现为空间电荷以包的形态沿着极化电场的方向进行迁移.目前针对空间电荷包现象的研究还存在一些不足,研究的对象通常集中在聚乙烯及其交联产物中的正极性空间电荷包.本文提出了一套用于负极性空间电荷包特性研究的一体化实验系统,可进行电子束辐照与压电压力波法空间电荷分布实时测量相结合的实验研究,并简要介绍了该系统的结构与功能.该系统适用于不同厚度范围的各类绝缘电介质样品在不同电场下的实验研究.本文使用该实验系统初步研究了在不同外加电场(15,20,2.5,30 kV/mm)下聚丙烯与聚甲基丙烯酸甲酯样品内负极性空间电荷包的迁移行为,并从实验结果中提取了负极性载流子;(电子)的迁移特性.聚丙烯与聚甲基丙烯酸甲酯样品中电子的迁移速率均存在随着电场的增加而减小的负微分迁移率现象,聚丙烯中该现象出现的阈值电场约为26.0 kV/mm,聚甲基丙烯酸甲酯中该现象出现的阈值电场约为19.5 kV/mm,消失的截止电场约为27.5 kV/mm.The space charge packet is a special sort of space charge phenomenon that is characterized by the migration of aggregated space charge in the form of a packet in the sample.Currently,most of the experimental and simulation studies on the generation and migration of space charge packets focus on the space charge packets with positive polarity in polyethylene and their cross-linking products,while the characteristics of the space charge packets with negative polarity still need studying.This paper presents an integrated experimental system for studying space charge packet with negative polarity,which enables experimental studies combining electron beam irradiation technique and real-time space charge distribution measurement.The beam flux for electron beam irradiation is controlled by a metal grid with an optical fiber-electric relay,and the space charge distribution measurement is performed by the piezo-pressure wave propagation method.The system achieves a withstand voltage value of 17 kV and a measuring resolution of 25 ns for space charge distribution measurement and is suitable for experimental studies of various material samples with different thickness ranges under different electric fields.In this work,the migration behaviors of space charge packets with negative polarity in polypropylene(PP)and polymethyl methacrylate(PMMA)samples under different applied electric fields(15,20,25,30 kV/mm)are studied by using the experimental system.The relationship between the migration properties of carriers with negative polarity(electrons)and the electric field can be extracted from the experimental results.The“negative differential mobility”phenomenon is found for both materials,i.e.the migration rate decreases with the increase of the electric field.The threshold electric field for the“negative differential mobility”phenomenon of electrons in PP sample is about 26.0 kV/mm while the threshold electric field for the“negative differential mobility”phenomenon of electrons in PMMA sample is 19.5 kV/mm,and the p

关 键 词：绝缘聚合物 空间电荷包 电子束辐照 载流子迁移率 

分 类 号：TM21[一般工业技术—材料科学与工程]