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机构地区:[1]Helmholtz Young Investigator Group Nanoscale Operando CO_(2)Photo-Electrocatalysis,Helmholtz-Zentrum Berlin für Materialien und Energie GmbH,Germany [2]Department of Interface Science,Fritz Haber Institute of the Max Planck Society,Germany
出 处:《National Science Review》2024年第7期59-60,共2页国家科学评论(英文版)
摘 要:By enabling the conversion of sustainably-derived electrical energy into chemical energy, electrocatalytic reactions are vital for closing the anthropogenic carbon cycle. A wide array of electrocatalytic reactions have gained extensive attention, including hydrogen evolution (HER), oxygen evolution (OER), and CO_(2) electroreduction (CO_(2)RR). However, progress in enhancing catalyst activity, selectivity, and stability is impeded by the lack of fundamental insight. Under reaction conditions, multi-step electron transfer and elementary catalytic processes convolute, influenced by the applied potential that affects the electrostatic potential of electrons through charging of the electric double layer (EDL) and/or the chemical potential of the electrocatalysts.
关 键 词:CATALYTIC ELECTRICAL ELEMENTARY
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