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作 者:Zhen Liu Li-Hua Wang Yong Jiang Ya-Jun Tong Hua-Chun Zhu Te Ji Min Chen Zheng Jiang Xiang-Jun Wei
机构地区:[1]Shanghai Advanced Research Institute,Chinese Academy of Sciences,Shanghai 201204,China [2]ShanghaiTech University,Shanghai 201210,China
出 处:《Nuclear Science and Techniques》2024年第9期56-67,共12页核技术(英文)
基 金:supported by the SSRF Phase-II Beamline Project.
摘 要:The dynamics beamline(D-Line),which combines synchrotron radiation infrared spectroscopy(SR-IR)and energy-disper-sive X-ray absorption spectroscopy(ED-XAS),is the first beamline in the world to realize concurrent ED-XAS and SR-IR measurements at the same sample position on a millisecond time-resolved scale.This combined technique is effective for investigating rapid structural changes in atoms,electrons,and molecules in complicated disorder systems,such as those used in physics,chemistry,materials science,and extreme conditions.Moreover,ED-XAS and SR-IR can be used independently in the two branches of the D-Line.The ED-XAS branch is the first ED-XAS beamline in China,which uses a tapered undulator light source and can achieve approximately 2.5×10^(12)photons/s·300 eV BW@7.2 keV at the sample position.An exchange-able polychromator operating in the Bragg-reflection or Laue-transmission configuration is used in different energy ranges to satisfy the requirements for beam size and energy resolution.The focused beam size is approximately 3.5μm(H)×21.5μm(V),and the X-ray energy range is 5–25 keV.Using one-and two-dimensional position-sensitive detectors with frame rates of up to 400 kHz enables time resolutions of tens of microseconds to be realized.Several distinctive techniques,such as the concurrent measurement of in situ ED-XAS and infrared spectroscopy,time-resolved ED-XAS,high-pressure ED-XAS,XMCD,and pump-probe ED-XAS,can be applied to achieve different scientific goals.
关 键 词:ED-XAS SR-IR TIME-RESOLVED D-line SSRF
分 类 号:TL594[核科学技术—核技术及应用]
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