面向PGNAA技术的碘化钠探测器MCNP模拟计算  

MCNP Simulation of NaI Detector for PGNAA Technology

作　　者：王泽亮 贾文宝[1] 杨晓艳 张镇华 张焱 程璨[1,4] WANG Zeliang;JIA Wenbao;YANG Xiaoyan;ZHANG Zhenhua;ZHANG Yan;CHENG Can(Nanjing University of Aeronautics and Astronautics,Nanjing 211106,China;Institute of Metrology and Testing of Inner Mongolia Autonomous Region,Hohhot 010030,China;East China University of Technology,Nanchang 330013,China;Nanjing University of Technology,Nanjing 210023,China)

机构地区：[1]南京航空航天大学,南京211106 [2]内蒙古自治区计量测试研究院,呼和浩特010030 [3]东华理工大学,南昌330013 [4]南京工业大学,南京210023

出　　处：《同位素》2024年第5期455-462,共8页Journal of Isotopes

基　　金：国家自然科学基金项目(12105143,42374226);国家重点研发计划(2023YFF0717003);江西省自然科学基金项目(2023BAB201043,20232BCJ23006);江苏省市场监督管理局科技计划项目(KJ2024009,KJ2024044,KJ2023015);放射医疗协同创新中心项目(YF202301)。

摘　　要：碘化钠(NaI)探测器因其优秀的探测效率和相对较低的成本在瞬发γ射线中子活化分析技术(prompt gamma-ray neutron activation analysis,PGNAA)中具有广泛应用。为了获取PGNAA测量过程中探测器对γ射线的响应,针对NaI探测器建立了蒙特卡罗模型,基于该模型对中子以及γ射线输运过程进行模拟计算。对^(60)Co、^(137)Cs、^(152)Eu、^(133)Ba和^(241)Am标准点源以及^(137)Cs水体源进行了测量分析,并与MCNP模拟计算进行对比,结果显示两者吻合。之后结合D-D中子发生器对水溶液进行测量,并分析H元素辐射俘获反应产生的2.223 MeV特征γ射线。研究结果表明,MCNP模拟计算的H元素特征峰计数与测量的结果偏差为13%,证明了MCNP建立的NaI测量系统模型能够实现对γ和中子混合输运过程的模拟仿真,可为后续系统优化工作的开展奠定基础。Sodium iodide(NaI) detector has wide applications in Prompt Gamma-ray Neutron Activation Analysis(PGNAA) due to its excellent detection efficiency and relatively low cost.In order to obtain the response of the detector to gamma-rays during PGNAA measurement process,a Monte Carlo model was established for the NaI detector to simulate the transport processes of neutrons and gamma-rays.Measurements and analyses were conducted on standard point sources of ^(60)Co,^(137)Cs,^(152)Eu,^(133)Ba,and ^(241)Am,as well as a waterborne source of ^(137)Cs.These measurements were compared with MCNP simulation calculations,and the results demonstrated agreement between the two methodologies.Then,measurements were conducted on aqueous solutions using a D-D neutron generator,and the 2.223 MeV characteristic gamma-ray produced by the H element radiative capture reaction was analyzed.The research results show that the deviations between MCNP simulation calculations of characteristic peaks for the H element and experimental measurements were consistently within 13%,demonstrating that the NaI measurement system model established by MCNP can simulate the transport processes of gamma and neutrons,laying a foundation for the subsequent optimization of the system and other related work.

关 键 词：NaI探测器 MCNP模拟 瞬发γ射线能谱 中子输运 

分 类 号：TL814[核科学技术—核技术及应用]