Highly efficient chemicalproductionviaelectrified,transient high-temperature synthesis  

作　　者：Yichen Dong Yi Rao Hanwen Liu Hao Zhang Rong Hu Yingquan Chen Yonggang Yao Haiping Yang 

机构地区：[1]State Key Laboratory of Coal Combustion,School of Energy and Power Engineering,Huazhong University of Science and Technology,Wuhan 430074,China [2]State Key Laboratory of Materials Processing and Die&Mould Technology,School of Materials Science and Engineering,Huazhong University of Science and Technology,Wuhan 430074,China

出　　处：《eScience》2024年第4期41-53,共13页电化学与能源科学（英文）

基　　金：The authors express their great appreciation for the support of National Natural Science Funds for Distinguished Young Scholar(52125601);Natural Science Foundation of Hubei Province,China(2022CFA031);the Open Fund of State Key Laboratory of New Textile Materials and Advanced Processing Technologies(FZ2022005);the Interdisciplinary Research Program of Huazhong University of Science and Technology(2023JCYJ004).

摘　　要：In response to the current energy and environmental challenges,reducing or replacing reliance on fossil fuels and striving for carbon neutrality seems to be the only viable choice.Recently,a cutting-edge,eco-friendly method of chemical synthesis via transient Joule heating(JH)demonstrated significant promise across various domains,including methane reforming,ammonia synthesis,volatile organic compounds removal,plastic recycling,the synthesis of functional carbon materials from repurposed solid waste,etc.In this review,the advantages,and latest developments in thermochemical synthesis by flash and transient JH are comprehensively outlined.Unlike the ongoing heating process of conventional furnaces that consume fossil fuels,dynamic and transient JH can get significantly higher reaction rates,energy efficiency,flexibility,and versatility.Subsequently,the transient reaction mechanism,data science optimization,and scale-up production models are discussed,and prospects for the integration of the electrified chemical industry with renewable energy for carbon neutrality and long-term energy storage are also envisioned.

关 键 词：Electrified chemicalsynthesis Transient heating Low-carbon production Gas-phasereaction Solid waste 

分 类 号：O62[理学—有机化学]