Ultrasonic enhancement of persulfate oxidation system governs emerging pollutants decontamination  

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作  者:Yanpan Li Yanbo Zhou Yi Zhou 

机构地区:[1]National Engineering Research Center of Industrial Wastewater Detoxication and Resource Recovery,State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process,East China University of Science and Technology,130 Meilong Road,Shanghai,200237,China [2]Shanghai Engineering Research Center for Multi-media Environmental Catalysis and Resource Utilization,East China University of Science and Technology,130 Meilong Road,Shanghai,200237,China [3]Shanghai Institute of Pollution Control and Ecological Security,Shanghai,200092,China

出  处:《Green Energy & Environment》2024年第11期1666-1678,共13页绿色能源与环境(英文版)

基  金:supported by the National Natural Science Foundation of China(No.22376065);Open Project of State Key Laboratory of Urban Water Resource and Environment,Harbin Institute of Technology(No.ESK202104);the Science and Technology Commission of Shanghai Municipality(22ZR1418600);Shanghai Municipal Science and Technology(No.20DZ2250400)

摘  要:Emerging contaminants (ECs) are widely present in aquatic environments, posing potential risks to both ecosystems and human health. Theultrasound-assisted persulfate oxidation process has attracted considerable attention in the degradation of ECs due to its ability to generate bothsulfate radicals and cavitation effects, enhancing degradation effects. In this paper, the principle of ultrasonic synergistic Fenton-like oxidationsystem for degrading organic pollutants was reviewed, divided into homogeneous system, non-homogeneous system, and single-atom system toexplore the synergistic effect of ultrasound-enhanced persulfate technology in three aspects, and the effects of environmental factors such asultrasonic frequency and power, system pH, temperature, and initial oxidant concentration on the system's decontamination performance werediscussed. Finally, future research on ultrasonically activated persulfate technology is summarized and prospected.

关 键 词:ULTRASOUND PERSULFATE Emerging contaminants Reaction mechanism Synergistic effects 

分 类 号:X505[环境科学与工程—环境工程]

 

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