金属有机骨架衍生碳基材料用于吸附-降解有机污染物的研究进展  

Advancement of metal-organic framework-derived carbon-based materials for adsorption-degradation of organic contaminants

作　　者：吴依璇 朱文君 李欣[1] 左小华 王浩南 Wu Yixuan;Zhu Wenjun;Li Xin;Zuo Xiaohua;Wang Haonan(Huangshihuli Environmental Protection and Energy Conservation Industry Technology Research Institute Co.,Ltd,College of Chemistry and Chemical Engineering,Hubei Polytechnic University,Huangshi 435003;Wuhan University of Technology,Wuhan 430070)

机构地区：[1]湖北理工学院化学与化工学院,黄石湖理环保节能产业技术研究院有限公司,黄石435003 [2]武汉理工大学,武汉430070

出　　处：《化工新型材料》2024年第S02期299-304,311,共7页New Chemical Materials

基　　金：国家自然科学基金(52072275);湖北理工学院大学生创新创业项目(S202210920008);湖北理工学院青年项目(22xjz01q);湖北理工学院人才引进项目(23xjz07R)。

摘　　要：随着人类社会发展,抗生素、内分泌干扰物以及染料等持久性有机化合物的频繁使用引发的水环境污染将对人体健康和生态环境造成不可逆的危害。因此,寻找绿色、高效和低成本的污染物处理技术刻不容缓。金属有机骨架(MOFs)衍生碳材料具有结构可控性强、比表面积大、化学稳定性高、表面可功能化等特点,在吸附-降解去除持久性有机污染物领域有着广泛应用。综述了MOFs衍生碳材料的制备过程、性质特点、阐述了其吸附-降解有机污染物的应用。最后探讨了MOFs衍生碳材料在水环境吸附-降解有机污染物应用中面临的挑战,并对其在吸附-降解有机污染物领域的未来研究和应用进行了展望。With the development of human society,the frequent use of persistent organic compounds such as antibiotics,endocrine disruptors,and dyes will result in the water pollution,which can cause irreversible harm to human health and the ecological environment.Therefore,it is urgent to explore green,efficient,and low-cost pollution treatment technologies.Metal-organic framework-derived carbon materials are characterized by strong structural controllability,large specific surface area,high chemical stability and surface functionalization,making them widely used in the field of adsorption-degradation for the removal of persistent organic contaminants.In this paper,the synthesis processes and property characteristics of MOFs-derived carbon materials were reviewed,and their application in the adsorption-degradation of organic contaminants were expounded.Finally,the challenges faced by MOFs-derived carbon materials in the application of adsorption-degradation of organic contaminants in aquatic environments were discussed,and their future research and application in the field of adsorption-degradation of organic contaminants were prospected.

关 键 词：有机污染物 废水处理 MOFs衍生碳材料 金属有机骨架 

分 类 号：TQ031.2[化学工程] X703[环境科学与工程—环境工程]