生化法处理城市污水一氧化二氮排放综述  

Review of Biochemical Treatment of N_(2)O Emissions from Urban Wastewater

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作  者:李清伟 程启原 郑家星 吴明松[1,2] LI Qing-wei;CHENG Qi-yuan;ZHENG Jia-xing;WU Ming-song(College of Resources and Civil Engineering,Northeastern University,Shenyang 110819,China;College of Resources and Materials,Northeastern University at Qinhuangdao,Qinhuangdao 066004,China)

机构地区:[1]东北大学资源与土木工程学院,沈阳110819 [2]东北大学秦皇岛分校资源与材料学院,秦皇岛066004

出  处:《科学技术与工程》2024年第32期13678-13687,共10页Science Technology and Engineering

基  金:中央高校基本科研业务专项(N2023031);河北省教育厅科学技术研究项目(ZC2021209)。

摘  要:“双碳”背景下,污水处理不仅要实现资源化,还要减少碳排放。为降低N_(2)O排放,中外学者对城镇污水厂N_(2)O排放开展了大量研究。首先,概述污水处理中硝化过程和反硝化过程都会产生N_(2)O,反应过程中产生N_(2)O机理与方式也存在差异,N_(2)O的产生量也会由于工艺不同而改变。其次,综述3种典型污水生物脱氮工艺:循环式活性污泥法(cyclic activated sludge system,CASS)工艺、厌氧氨氧化(anaerobic ammonium oxidation,ANAMMOX)工艺、亚硝化-厌氧氨氧化(nitrosation anaerobic ammonium oxidation,CANON)工艺,以及影响城镇污水厂N_(2)O排放量产生的4种因素:碳源、溶解氧浓度、温度、磁场强度。最后,总结目前研究尚存在的不足,并从温度影响条件、碳源种类、CANON工艺机理、N_(2)O回收利用4个方面进行展望。CANON工艺对于去除N_(2)O有较好的效果,但需注意,反应中PH过低使NH 2OH和HNO 2反应生成N_(2)O,从而削弱去除效果。Under the background of“dual carbon”,sewage treatment not only needs to achieve resource utilization,but also needs to reduce carbon emissions.To reduce N_(2)O emissions,scholars at home and abroad have conducted extensive research on N_(2)O emissions from urban sewage plants.Firstly,it was summarized that both nitrification and denitrification processes in wastewater treatment produce N_(2)O.The mechanism and mode of N_(2)O production during the reaction process also differ,and the amount of N_(2)O produced may vary depending on the process.Secondly,three typical biological denitrification processes for wastewater were reviewed:cyclic activated sludge system(CASS)process,anaerobic ammonium oxidation(ANAMMOX)process,and nitrosation anaerobic ammonium oxidation(CANON)process,as well as four factors affecting N_(2)O emissions from urban wastewater treatment plants:carbon source,dissolved oxygen concentration,temperature,and magnetic field strength.Finally,the shortcomings of current research were summarized and provided prospects from four aspects:temperature influencing conditions,carbon source types,CANON process mechanisms,and N_(2)O recovery and utilization.The CANON process is effective for removing N_(2)O,but it should be noted that a low pH in the reaction can cause NH 2OH and HNO 2 to react and produce N_(2)O,thereby weakening the removal effect.

关 键 词:双碳 硝化 N_(2)O 反硝化 碳源 

分 类 号:X511[环境科学与工程—环境工程]

 

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