The strategies to improve TMDs represented by MoS_(2)electrocatalytic oxygen evolution reaction  

作　　者：Junan Pan Xinyi Liu Huachao Ji Yanwei Zhu Yanling Zhuang Kang Chen Ning Sun Yongqi Liu Yunchao Lei Kun Wang Bao Zang Longlu Wang 

机构地区：[1]State Key Laboratory of Organic Electronics and Information Displays&Jiangsu Key Laboratory for Biosensors,College of Electronic and Optical Engineering&College of Flexible Electronics(Future Technology),Nanjing 210023,China [2]State Key Laboratory of Chemo/Bio-Sensing and Chemometrics,College of Chemistry and Chemical Engineering,Advanced Catalytic Engineering Research Center of the Ministry of Education,Hunan University,Changsha 410082,China

出　　处：《Chinese Chemical Letters》2024年第11期203-213,共11页中国化学快报（英文版）

基　　金：financially supported by the National Natural Science Foundation of China(No.51902101);Natural Science Foundation of Jiangsu Province(No.BK20201381);Science Foundation of Nanjing University of Posts and Telecommunications(No.NY219144);the National College Student Innovation and Entrepreneurship Training Program(No.202310293173K)。

摘　　要：The hydrogen evolution reaction(HER)and the oxygen evolution reaction(OER)are the two half reactions that make up the over water splitting reaction.Increasing oxygen evolution reaction rate wound immensely raise the efficiency of over water splitting reaction because it is the rate limiting reaction in water splitting reaction.The key to improve OER performance is the development and utilization of advanced catalysts.As one of the most potential catalysts for HER,it has gradually attracted the attention of researchers in the aspect of catalytic OER.It is very necessary to review the research progress of Transition metal dichalcogenides(TMDs)in catalytic OER to promote the research process in the field.In this review,we comprehensively and systematically summarized the strategies to improve TMDs electrocatalytic OER.First of all,structural regulation of TMDs-based electrocatalyst was summarized in detail,mainly including size engineering,defect engineering,doping engineering,phase engineering and heterojunction engineering.Once more,magnetic field regulation as a representative of external field regulation to improve TMDs electrocatalytic OER performance was discussed in depth.Last but not least,the strategies to improve TMDs electrocatalytic OER is prospected and some views on the development of this field are also put forward,which are expected to enhance the catalytic efficiency of TMDs for OER.

关 键 词：Oxygen evolution reaction Transition metal dichalcogenides Structural regulation External field regulation ELECTROCATALYST 

分 类 号：O643.36[理学—物理化学]