Aqueous Zn-CO_(2) batteries:a route towards sustainable energy storage  

作　　者：Yanxiu Liu Junjie Chen Weichen Li Yu Zhang Xianwei Fu Erling Li Shangbin Jin Li-Ming Yang Zhihong Tian Markus Antonietti Tianxi Liu 

机构地区：[1]School of Mechanical and Power Engineering,East China University of Science and Technology,Shanghai 200237,China [2]Engineering Research Center for Nanomaterials,Henan University,Kaifeng 475004,P.R.China [3]Department of Colloid Chemistry,Max Planck Institute of Colloids and Interfaces,Potsdam 14476,Germany [4]Key Laboratory of Synthetic and Biological Colloids,Ministry of Education,School of Chemical and Material Engineering,Jiangnan University,Wuxi 214122,P.R.China [5]School of Chemical Engineering and Technology,Xi'an Jiaotong University,28 Xianning Road,Xi'an,Shaanxi,710049,China [6]School of Chemistry and Chemical Engineering,Huazhong University of Science and Technology,Wuhan 430074,China

出　　处：《Industrial Chemistry & Materials》2024年第4期514-532,共19页工业化学与材料（英文）

基　　金：This work was supported by the National Natural Science Foundation of China(No.22109044,52373205,52003251,52102166);Natural Science Foundation of Shanghai,China(No.22ZR1418500);start-up funds from the East China University of Science and Technology,and Henan Center for Outstanding Overseas Scientists(GZS2022014).

摘　　要：In recent years,the concept of rechargeable aqueous Zn–CO_(2) batteries has attracted extensive attention owing to their dual functionality of power supply and simultaneous conversion of CO_(2) into value-added chemicals or fuels.The state-of-the-art research has been mainly focused on the exploration of working mechanisms and catalytic cathodes but hardly applies an integrative view.Although numerous studies have proven the feasibility of rechargeable aqueous Zn–CO_(2) batteries,challenges remain including the low CO_(2) conversion efficiency,poor battery capacity,and low energy efficiency.This review systematically summarizes the working principles and devices,and the catalytic cathodes used for Zn–CO_(2) batteries.The challenges and prospects in this field are also elaborated,providing insightful guidance for the future development of rechargeable aqueous Zn–CO_(2) batteries with high performance.

关 键 词：Zn-CO_(2)battery CO_(2)reduction reaction Working mechanism ELECTROCATALYSTS 

分 类 号：TM9[电气工程—电力电子与电力传动]