Recent progress in nickel single-atom catalysts for the electroreduction of CO_(2) to CO  

作　　者：Ziyan Yang Rongzhen Chen Ling Zhang Yuhang Li Chunzhong Li 

机构地区：[1]Key Laboratory for Ultrafine Materials of Ministry of Education,Shanghai Engineering Research Center of Hierarchical Nanomaterials,School of Materials Science and Engineering,East China University of Science and Technology,Shanghai 200237,People's Republic of China [2]Key Laboratory for Ultrafine Materials of Ministry of Education,Shanghai Engineering Research Center of Hierarchical Nanomaterials,School of Chemical Engineering,East China University of Science and Technology,Shanghai 200237,People's Republic of China

出　　处：《Industrial Chemistry & Materials》2024年第4期533-555,共23页工业化学与材料（英文）

基　　金：This work was supported by the National Natural Science Foundation of China(22322805,22178104,U22B20143);Shanghai Municipal Science and Technology Major Project,the Shanghai Scientific and Technological Innovation Project(22dz1205900);“the Fundamental Research Funds for the Central Universities”;Shanghai Rising-Star Program(23QA1402200).

摘　　要：The electrocatalytic reduction of carbon dioxide(CO_(2))is considered an effective strategy for mitigating the energy crisis and the greenhouse effect.Nickel is widely used in single-atom catalysts(SACs)owing to its special electronic structure.In this minireview,the basic principles of Ni SACs in the electrocatalytic reduction of CO_(2) to CO are first described.Subsequently,Ni SACs are divided into three categories depending on different strategies used to improve properties.The synthesis,morphology,performance and theoretical calculations of the catalysts are also described.Finally,an overview of the existing challenges and perspectives of Ni SACs for CO_(2) reduction is presented.

关 键 词：CO_(2)reduction ELECTROCATALYSIS Nickel single-atom catalysts 

分 类 号：O64[理学—物理化学]