太阳能驱动的无机半导体-微生物杂化体系在二氧化碳固定和生物制造中的应用  

Application of solar⁃driven inorganic semiconductor⁃microbe hybrids in carbon dioxide fixation and biomanufacturing

作　　者：何为 席京 贺天培 陈娜 袁荃 HE Wei;XI Jing;HE Tianpei;CHEN Na;YUAN Quan(Renmin Hospital of Wuhan University,Wuhan 430060,China;College of Chemistry and Molecular Sciences,Wuhan University,Wuhan 430072,China)

机构地区：[1]武汉大学人民医院,武汉430060 [2]武汉大学化学与分子科学学院,武汉430072

出　　处：《无机化学学报》2025年第1期35-44,共10页Chinese Journal of Inorganic Chemistry

基　　金：国家自然科学基金(No.21925401);中国博士后科学基金(No.2024M752456);湖北省博士后创新研究项目(No.211000025);中国科协智库青年人才项目(No.XMSB20240710060);武汉大学人民医院交叉创新人才项目资助。

摘　　要：随着全球经济的快速发展,传统化石能源消耗显著增加,导致了二氧化碳(CO_(2))的大量排放,这对自然生态造成了显著的影响。近年来,由太阳能驱动的以大气中CO_(2)为原料的第3代绿色生物制造技术引起了全球广泛关注。过去数年间,研究者们在太阳能驱动的无机半导体-微生物杂化体系领域开展了大量的工作,这对CO_(2)固定以及生物制造领域具有深远的影响。本综述围绕如何构筑高性能无机半导体-微生物杂化体系,分别从无机半导体材料的结构性能优化、无机半导体-微生物界面的构筑以及微生物代谢通路的定向重构3个维度进行了全面综述。最后,本综述展望了无机半导体-微生物杂化体系领域的发展趋势。As the global economy develops rapidly,the consumption of traditional fossil fuels has significantly increased,leading to a substantial emission of carbon dioxide(CO_(2)),which has a noticeable impact on the natural ecosystem.In recent years,the third‑generation green bio‑manufacturing technology,driven by solar energy and using atmospheric CO_(2)as raw material,has gained widespread global attention.Over the past several years,researchers have conducted extensive studies in solar‑driven inorganic semiconductor‑microorganism hybrid systems,which have profound implications for CO_(2)fixation and bio‑manufacturing.This review comprehensively examines how to construct high‑performance inorganic semiconductor‑microorganism hybrid systems by focusing on three dimensions:the optimization of inorganic semiconductor material structures and properties,the construction of inorganic semiconductor‑microorganism interfaces,and the targeted reconstruction of microorganism metabolic pathways.Finally,this review outlines the developmental trends in the field of inorganic semiconductor‑microorganism hybrid systems.

关 键 词：半导体-微生物杂化体系 CO_(2)固定 生物制造 

分 类 号：TN304.9[电子电信—物理电子学] Q936[生物学—微生物学]