机构地区:[1]Center for Carbon-based Electronics and Key Laboratory for the Physics and Chemistry of Nanodevices,School of Electronics,Peking University,Beijing 100871,China [2]Spin-X Institute,School of Microelectronics,South China University of Technology,Guangzhou 511442,China [3]School of Materials and Energy,Guangzhou Key Laboratory of Low-Dimensional Materials and Energy Storage Devices,Guangdong University of Technology,Guangzhou 510006,China [4]Faculty of Materials Science and Engineering,Kunming University of Science and Technology,Kunming 650093,China [5]i-Lab,CAS Key Laboratory of Nanophotonic Materials and Devices,Suzhou Institute of Nano-Tech and Nano-Bionics,Chinese Academy of Sciences,Suzhou 215123,China [6]CAS Key Laboratory of Molecular Nanostructure and Nanotechnology,CAS Research/Education Center for Excellence in Molecular Sciences,Beijing National Laboratory for Molecular Sciences(BNLMS),Institute of Chemistry,Chinese Academy of Sciences,Beijing 100190,China [7]State Key Laboratory for Organic Electronics and Information Displays&Jiangsu Key Laboratory for Biosensors,Institute of Advanced Materials,Jiangsu National Synergetic Innovation Center for Advanced Materials,Nanjing University of Posts and Telecommunications,Nanjing 210023,China [8]Institute of Functional Nano and Soft Materials(FUNSOM),Jiangsu Key Laboratory for Carbon-Based Functional Materials and Devices,Soochow University,Suzhou 215123,China [9]Hefei National Research Center for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information and Quantum Physics,University of Science and Technology of China,Hefei 230026,China [10]Institute of Physics&University of Chinese Academy of Sciences,Beijing 100190,China [11]State Key Laboratory of Catalysis,Dalian Institute of Chemical Physics,Chinese Academy of Sciences,Dalian 116023,China [12]College of Chemistry,Beijing Normal University,Beijing 100875,China [13]Beijing National Laboratory for Molecular Sciences(BNLMS),College of Chemistry and Molecular Engineering,Pe
出 处:《Chinese Chemical Letters》2025年第1期8-57,共50页中国化学快报(英文版)
摘 要:Surface with well-defined components and structures possesses unique electronic,magnetic,optical and chemical properties.As a result,surface chemistry research plays a crucial role in various fields such as catalysis,energy,materials,quantum,and microelectronics.Surface science mainly investigates the correspondence between surface property and functionality.Scanning probe microscopy(SPM)techniques are important tools to characterize surface properties because of the capability of atomic-scale imaging,spectroscopy and manipulation at the single-atom level.In this review,we summarize recent advances in surface electronic,magnetic and optical properties characterized mainly by SPM-based methods.We focus on elucidating theπ-magnetism in graphene-based nanostructures,construction of spin qubits on surfaces,topology properties of surface organic structures,STM-based light emission,tip-enhanced Raman spectroscopy and integration of machine learning in SPM studies.
关 键 词:Surface chemistry Scanning probe microscopy π-Magnetism Spin qubits Tip-enhanced Raman spectroscopy
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