High summer background O_(3)levels in the desert of northwest China  

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作  者:Xinbing Ren Fang Wang Bayi Wu Shaoting Zhang Lei Zhang Xingjun Zhou Yuanzhe Ren Yongjing Ma Feng Hao Yongli Tian Jinyuan Xin 

机构地区:[1]Key Laboratory of Atmospheric Environment and Extreme Meteorology,Institute of Atmospheric Physics,Chinese Academy of Sciences,Beijing 100029,China [2]State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry(LAPC),Institute of Atmospheric Physics,Chinese Academy of Sciences,Beijing 100029,China [3]College of Earth and Planetary Sciences,University of Chinese Academy of Sciences,Beijing 100049,China [4]Inner Mongolia Environmental Monitoring Center,Alashan Substation 750300,China [5]Inner Mongolia Environmental Monitoring Center,Hohhot 010011,China [6]Laboratory for Supervision and Evaluation of Pollution Reduction and Carbon Reduction in Arid and Semi-Arid Regions,Inner Mongolia Environmental Monitoring Center,Hohhot 010011,China

出  处:《Journal of Environmental Sciences》2025年第5期516-528,共13页环境科学学报(英文版)

基  金:supported by the Ministry of Science and Technology of China(No.2022YFF0802501);Inner Mongolia Autonomous Region Science and Technology Program(Nos.2021GG0100 and 2022YFHH0116).

摘  要:Generally speaking,the precursors of ozone(O_(3)),nitrogen oxides and volatile organic compounds are very low in desert areas due to the lack of anthropogenic emissions and natural emissions,and thus O_(3)concentrations are relatively low.However,high summer background concentrations of about 100μg/m^(3)or 60 ppb were found in the Alxa Desert in the highland of northwest China based on continuous summer observations from 2019 to 2021,which was higher than the most of natural background areas or clean areas in world for summer O_(3)background concentrations.The high O_(3)background concentrations were related to surface features and altitude.Heavy-intensity anthropogenic activity areas in desert areas can cause increased O_(3)concentrations or pollution,but also generated O_(3)depleting substances such as nitrous oxide,which eventually reduced the regional O_(3)baseline values.Nitrogen dioxide(NO2)also had a dual effect on O_(3)generation,showing promotion at low concentrations and inhibition at high concentrations.In addition,sand-dust weather reduced O_(3)clearly,but O_(3)eventually stabilized around the background concentration values and did not vary with sand-dust particulate matter.

关 键 词:Alxa Desert O_(3)background concentration Anthropogenic effect Sand-dust weather Northwest China 

分 类 号:X515[环境科学与工程—环境工程]

 

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