Green innovation unleashed:Harnessing tungsten-based nanomaterials for catalyzing solar-driven carbon dioxide conversion  

作　　者：Weidan Meng Yanbo Zhou Yi Zhou 

机构地区：[1]State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process,East China University of Science and Technology,Shanghai 200237,China [2]National Engineering Research Center of Industrial Wastewater Detoxication and Resource Recovery,East China University of Science and Technology,Shanghai 200237,China [3]Shanghai Engineering Research Center for Multi-media Environmental Catalysis and Resource Utilization,East China University of Science and Technology,Shanghai 200237,China [4]Shanghai Institute of Pollution Control and Ecological Security,Shanghai 200092,China

出　　处：《Chinese Chemical Letters》2025年第2期108-117,共10页中国化学快报(英文版)

基　　金：supported by the National Natural Science Foundation of China(No.22376065);the Science and Technology Commission of Shanghai Municipality(No.22ZR1418600);Shanghai Municipal Science and Technology(No.20DZ2250400)。

摘　　要：Carbon dioxide photocatalytic reduction (CO_(2)-PR) is an efficient method for controlling CO_(2)emissions and generating cleaner energy while mitigating global warming.Tungsten oxides (WxOy) have attracted considerable attention for CO_(2)-PR due to their excellent spectral absorbance.However,comprehensive reviews are lacking on the use of WxOyfor CO_(2)-PR.Therefore,this review provides a detailed summary of t research progress made with WxOy-based catalysts in CO_(2)-PR.It also explains the fundamental principles of CO_(2)-PR and evaluates key performance indicators that affect the activity of WxOy-based photocatalysts,including yield,selectivity,stability,and apparent quantum yield.Additionally,this review explores opportunities for synthesizing high-performance WxOy-based photocatalysts and highlights their potential for the green preparation of C1/C2 products through CO_(2)-PR.These innovative strategies aim to address the challenges and pressures associated with energy and environmental issues,particularly by enhancing artificial photosynthesis efficiency.

关 键 词：Carbon dioxide photoreduction Tungsten-based nanocatalyst Mechanism Performance evaluation Selectivity 

分 类 号：X701[环境科学与工程—环境工程] O643.36[理学—物理化学] O644.1[理学—化学]