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作 者:杨晋宁 王卫凡 徐冬 刘毅 翁小涵 原野 王志[2] YANG Jinning;WANG Weifan;XU Dong;LIU Yi;WENG Xiaohan;YUAN Ye;WANG Zhi(National Energy Group New Energy Technology Research Institute Co.,Ltd.,Beijing 102209,China;Chemical Engineering Research Center,School of Chemical Engineering and Technology(Tianjin University),Tianjin Key Laboratory of Membrane Science and Desalination Technology,State Key Laboratory of Chemical Engineering(Tianjin University),Tianjin Collaborative Innovation Center of Chemical Science and Engineering,Tianjin 300350,China)
机构地区:[1]国家能源集团新能源技术研究院有限公司,北京102209 [2]天津大学化工学院化学工程研究所,天津市膜科学与海水淡化技术重点实验室,化学工程联合国家重点实验室(天津大学),天津化学化工协同创新中心,天津300350
出 处:《化工学报》2025年第2期504-518,共15页CIESC Journal
基 金:国家能源集团科技项目(GJNY-23-88)。
摘 要:工业烟道气是全球碳排放的主要来源之一,也是碳捕集技术的重点应用领域。综述了工业烟道气碳捕集领域中的膜技术放大研究进展。首先,介绍了CO_(2)/N_(2)分离膜的工作原理。其次,总结了化石能源发电厂、水泥厂、钢铁厂烟道气的来源与成分,并分析了在这些烟道气碳捕集过程中膜分离技术所面临的挑战。然后,对烟道气碳捕集膜的放大生产、烟道气碳捕集膜组件研究、工业烟道气碳捕集膜放大测试进行现状介绍和问题分析。最后,展望了膜技术在工业烟道气碳捕集中的发展方向,包括实现CO_(2)分离混合基质膜放大、针对钢铁厂烟道气的CO分离膜的开发以及膜组件的优化。旨在为学者们提供工业烟气碳捕捉膜放大的最新研究进展和未来方向。CO_(2)emissions from industrial flue gases are among the primary sources of global carbon emissions and are key areas for the application of carbon capture technologies.The research progress on scale-up of membrane technology in the field of carbon capture from industrial flue gas is reviewed.First,the working principles of CO_(2)/N_(2)separation membranes are introduced.The sources and compositions of flue gases from fossil fuel power plants,cement plants,and steel plants are summarized,and the challenges faced by membrane separation technology in the carbon capture process of these flue gases are discussed.Next,the current status and issues related to the scale-up preparation of flue gas carbon capture membranes,research on flue gas carbon capture membrane modules,and scale-up testing of industrial flue gas carbon capture membranes are introduced and analyzed.Finally,the development trends in membrane technology for industrial flue gas carbon capture are discussed,including the scale-up of CO_(2)separation mixed-matrix membranes,the development of CO separation membranes for steel mill flue gases,and the optimization of membrane modules.This review aims to provide scholars with the latest research developments and future directions in the scale-up of industrial flue gas carbon capture membranes.
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