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作 者:Yuchen Zhang Lifeng Ding Zhenghe Xie Xin Zhang Xiaofeng Sui Jian-Rong Li
机构地区:[1]Beijing Key Laboratory for Green Catalysis and Separation and Department of Chemical Engineering,College of Materials Science&Engineering,Beijing University of Technology,Beijing 100124,China [2]Beijing Energy Holding Company Limited,Beijing 100022,China
出 处:《Chinese Chemical Letters》2025年第3期125-133,共9页中国化学快报(英文版)
基 金:financial support from the National Natural Science Foundation of China(Nos.22278011,22225803,22038001 and 22108007);Beijing Natural Science Foundation(No.Z230023);The Science&Technology Project of Beijing Municipal Education Committee(No.KZ201810005004);Beijing Nova Program(No.Z211100002121094)。
摘 要:Large-scale deployment of carbon dioxide(CO_(2))removal technology is an essential step to cope with global warming and achieve carbon neutrality.Direct air capture(DAC)has recently received increasing attention given the high flexibility to remove CO_(2)from discrete sources.Porous materials with adjustable pore characteristics are promising sorbents with low or no latent heat of vaporization.This review article has summarized the recent development of porous sorbents for DAC,with a focus of pore engineering strategy and adsorption mechanism.Physisorbents such as zeolites,porous carbons,metal-organic frameworks(MOFs),and amine-modified chemisorbents have been discussed and their challenges in practical application have been analyzed.At last,future directions have been proposed,and it is expected to inspire collaborations from chemistry,environment,material science and engineering communities.
关 键 词:Direct air capture Carbon neutrality Porous materials PHYSISORPTION CHEMISORPTION
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