燃烧后CO_(2)捕集固体吸附剂研究进展  

Research progress of solid adsorbents for CO_(2)capture after combustion

作　　者：卓华伟 李芹 梅雪丽 徐博凡 谢洪涛 耿芹 李怡招 ZHUO Huawei;LI Qin;MEI Xueli;XU Bofan;XIE Hongtao;GENG Qin;LI Yizhao(Yangtze Delta Region Institute(Huzhou),University of Electronic Science and Technology of China,Huzhou 313001,Zhejiang Province,China;College of Chemical Engineering,Xinjiang University,Urumchi 830046,Xinjiang,China;Huzhou Environmental Protection Group Co.,Ltd.,Huzhou 313000,Zhejiang Province,China)

机构地区：[1]电子科技大学长三角研究院(湖州),浙江湖州313001 [2]新疆大学化工学院,新疆乌鲁木齐830046 [3]湖州市环保集团有限公司,浙江湖州313000

出　　处：《化学工程》2025年第4期89-94,共6页Chemical Engineering(China)

基　　金：浙江省“尖兵”“领雁”研发攻关计划项目(2023C03017);国家自然科学基金资助项目(52100166,22306023)。

摘　　要：为应对大气中CO_(2)浓度逐年攀升的挑战,燃烧后CO_(2)捕集技术展现出广阔的应用前景。综述燃烧后CO_(2)捕集技术的多种方法,重点探讨固体吸附剂的应用和发展。首先,阐述4种主流方法的原理及工艺,包括吸收法、膜分离法、低温分离法和吸附法。随后,聚焦于固体吸附剂,探讨多孔碳基吸附剂、沸石、MOFs(金属有机骨架)和SiO 2的最新研究进展。通过分析这些吸附剂的结构和性能,探讨它们在CO_(2)捕集领域的优势和挑战。最后,对固体吸附剂的未来发展进行展望,指出其在许多方面仍存在广阔的研究空间和创新机遇。随着技术进步和研究的深入,固体吸附剂在CO_(2)捕集领域的应用将更加广泛,为实现双碳目标和可持续发展提供有力支持。In light of the ongoing increase in atmospheric CO_(2)concentration,the potential for CO_(2)capture after combustion technology shows a broad application prospect.Various methods of CO_(2)capture technology were reviewed with a specific focus on the application and development of solid adsorbents.Firstly,the principles and processes of four mainstream methods of CO_(2)capture technology were described,including absorption,membrane separation,low temperature separation and adsorption.Then,focusing on solid adsorbents,the latest research progress of porous carbon-based adsorbents,zeolites,MOFs(metal-organic frameworks)and SiO 2 was discussed.The advantages and challenges of these adsorbents in the field of CO_(2)capture were explored through an analysis of their structures and properties.Finally,the future development of solid adsorbents was prospected,indicating that there was still a broad research space and innovative opportunities in many aspects.As a consequence of technological progress and in-depth research,the application of solid adsorbents in the field of CO_(2)capture will become more extensive,thereby providing strong support for the realization of the dual-carbon goal and sustainable development.

关 键 词：燃烧后CO_(2)捕集技术 吸附法 固体吸附剂 

分 类 号：TQ424[化学工程] O6.1[理学—化学]