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作 者:张新新 岑官骏 乔荣涵 朱璟 郝峻丰 孙蔷馥 田孟羽 金周 詹元杰 闫勇 贲留斌 俞海龙[1] 刘燕燕[1] 周洪[3] 黄学杰[1,2] ZHANG Xinxin;CEN Guanjun;QIAO Ronghan;ZHU Jing;HAO Junfeng;SUN Qiangfu;TIAN Mengyu;JIN Zhou;ZHAN Yuanjie;YAN Yong;BEN Liubin;YU Hailong;LIU Yanyan;ZHOU Hong;HUANG Xuejie(Institute of Physics,Chinese Academy of Sciences,Beijing 100190,China;Songshan Lake Materials Laboratory,Dongguan 523890,Guangdong,China;National Science Library(Wuhan),Chinese Academy of Sciences,Wuhan 430071,Hubei,China)
机构地区:[1]中国科学院物理研究所,北京100190 [2]松山湖材料实验室,广东东莞523890 [3]中国科学院武汉文献情报中心,湖北武汉430071
出 处:《储能科学与技术》2025年第3期1310-1329,共20页Energy Storage Science and Technology
摘 要:文本,构建锂电池论文的研究主题图,再选择其中100篇加以评论。正极材料的研究集中于高镍层状材料和尖晶石结构LiNi_(0.5)Mn_(1.5)O_(4)材料的掺杂改性、表面包覆、结构设计等。负极材料的研究重点包括硅基负极的结构设计和性能提升、金属锂负极的界面和体相结构设计。固态电解质的研究包括对聚合物、硫化物和卤化物及其复合固态电解质的结构设计以及相关性能研究。其他电解液和添加剂的研究则主要包括不同电解质和溶剂对各类电池材料体系适配的研究,以及对新的功能性添加剂的探索。对固态电池,正极材料的体相改性、表面包覆和合成方法、锂金属负极的界面构筑和三维结构设计、无负极集流体的界面修饰有多篇文献报道。此外,锂硫电池和锂空电池也备受关注。电极中的锂离子输运和失效机制、锂沉积形貌和SEI结构演变、全电池热失控分析,电解质对CEI组分影响的理论模拟以及优化制造工艺的论文也有多篇。This bimonthly review provides a comprehensive overview of recent research on lithium batteries.A total of 5413 online papers published between December 1,2024 and January 31,2025 were examined using the Web of Science database.Using the BERTopic model,the abstract texts were analyzed,and a research topic map for lithium battery studies was generated.From these,100 papers were selected for in-depth discussion.The selected studies covered various aspects of lithium batteries.Research on cathode materials,including Ni-rich layered oxides and LiNi_(0.5)Mn_(1.5)O_(4),focuses on improvements through doping,surface coating,and microstructural modifications.The cycling performances of Si-based anodes were enhanced through structural design.Considerable efforts have been devoted to interfacial and bulk structure design for lithium metal anodes.Studies on solid-state electrolytes examined structural design and performance in polymer,sulfide,and halide electrolytes as well as their composite forms.In contrast,liquid electrolytes were improved through optimized solvent and lithium salt designs for different battery applications and the incorporation of novel functional additives.For solid-state batteries,studies have explored cathode modification,surface coating,and synthesis methods as well as interface construction and three-dimensional structural design for lithium metal anodes.Interface modifications of current collectors for anode-free batteries have also been widely investigated.In lithium-sulfur batteries,the structural design of the cathode and liquid electrolyte contributes to extended cycle life.In addition,lithium-sulfur and lithium-oxygen batteries have garnered considerable attention.Other studies have investigated ion transport and degradation mechanisms in electrodes,lithium deposition morphology,and solid electrolyte interphase evolution.Research has also addressed thermal runaway analysis in full batteries,theoretical simulations of solvent effects on the cathode electrolyte interphase,and optimization of m
分 类 号:TM911[电气工程—电力电子与电力传动]
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