Inorganic chemical composition and source signature of PM2.5 in Beijing during ACE-Asia period  

作　　者：ZHANG Renjian, XU Yongfu & HAN Zhiwei LAPC, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China 

出　　处：《Chinese Science Bulletin》2003年第10期1002-1005,共4页

基　　金：supported by the National Natural Science Foundation of China(Grant No.40205017);the Knowledge Innovation Project(Grant No.KZCX2-305);Hundred Talents Program(Global Environmental Change)by the Chinese Academy of Sciences.

摘　　要：Aerosol samples for PM2.5 were collected in Beijing for 38 consecutive days from March to April 2001 using an IMPROVE Sampler. Concentrations of 20 elements in PM2.5 were determined using a PIXE method. Results show that the average mineral dust concentration of PM2.5 was 14.6 mg/m3 during the observation period. On the sand-dust event days of March 21 and April 10, dust PM2.5 mass concentrations were 62.4 and 54.1 mg/m3, respectively. These demonstrate that fine particle pollution by dust event in Beijing was very severe. The enrichment factors of S and Cu reached minimums on the dusty days and were high on the non-dusty days. It is considered that enrichment factors of elements in PM2.5, which are associated with human activities, can probably provide an effective method to distinguish local sources from external sources of dust. Factor analysis on the chemical composition in PM2.5 shows that sources of crustal matters, anthropogenic emission, and oil combustion contributed to PM2.5 levels in air in the springtime of 2001 in Beijing.Aerosol samples for PM2.5 were collected in Beijing for 38 consecutive days from March to April 2001 using an IMPROVE Sampler. Concentrations of 20 elements in PM2.5 were determined using a PIXE method. Results show that the average mineral dust concentration of PM2.5 was 14.6 mg/m3 during the observation period. On the sand-dust event days of March 21 and April 10, dust PM2.5 mass concentrations were 62.4 and 54.1 mg/m3, respectively. These demonstrate that fine particle pollution by dust event in Beijing was very severe. The enrichment factors of S and Cu reached minimums on the dusty days and were high on the non-dusty days. It is considered that enrichment factors of elements in PM2.5, which are associated with human activities, can probably provide an effective method to distinguish local sources from external sources of dust. Factor analysis on the chemical composition in PM2.5 shows that sources of crustal matters, anthropogenic emission, and oil combustion contributed to PM2.5 levels in air in the springtime of 2001 in Beijing.

关 键 词：无机化学 化合物 PM2.5 起源 铀 大气成分 灰尘 污染物质 

分 类 号：X831[环境科学与工程—环境工程]