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High Fe‑Loading Single‑Atom Catalyst Boosts ROS Production by Density Effect for Efficient Antibacterial Therapy
《Nano-Micro Letters》2025年第2期187-203,共17页Si Chen Fang Huang Lijie Mao Zhimin Zhang Han Lin Qixin Yan Xiangyu Lu Jianlin Shi 
supported by the National Key Research and Development Program of China(Grant No.2022YFB3804500);the National Natural Science Foundation of China(Grant No.52202352,22335006);the Shanghai Municipal Health Commission(Grant No.20224Y0010);the CAMS Innovation Fund for Medical Sciences(Grant No.2021-I2M-5-012);the Basic Research Program of Shanghai Municipal Government(Grant No.21JC1406000);the Fundamental Research Funds for the Central Universities(Grant No.22120230237,2023-3-YB-11,22120220618);the Basic Research Program of Shanghai Municipal Government(23DX1900200).
The current single-atom catalysts(SACs)for medicine still suffer from the limited active site density.Here,we develop a synthetic method capable of increasing both the metal loading and mass-specific activity of SACs ...
关键词：Nanocatalytic medicine Single-atom catalysts Reactive oxygen species(ROS) High metal loading Oxidase catalysis 
Rational design of MXene-based vacancy-confined single-atom catalyst for efficient oxygen evolution reaction
《Journal of Energy Chemistry》2024年第11期663-669,共7页Zhongheng Fu Guangtong Hai Xia-Xia Ma Dominik Legut Yongchao Zheng Xiang Chen 
National Natural Science Foundation of China (22209094, 22209093);Research Funds of Institute of Zhejiang University-Quzhou (No. IZQ2023RCZX032);USTB Mat Com of Beijing Advanced Innovation Center for Materials Genome Engineering;Ministry of Education, Youth and Sports of the Czech Republic through the e-INFRA CZ (ID:90254);project Quantum materials for applications in sustainable technologies (QM4ST), funded as project No. CZ.02.01.01 /00/22_008/0004572。
Two-dimensional transition metal carbides(MXenes) have been demonstrated to be promising supports for single-atom catalysts(SACs) to enable efficient oxygen evolution reaction(OER).However,the rational design of MXene...
关键词：MXene Single-atom catalysis Oxygen evolution reaction High-throughput calculation Machine learning 
Theoretical and experimental investigations on single-atom catalysis:Pt_(1)/FeO_(x) for water-gas shift reaction
《Nano Research》2024年第9期8627-8637,共11页Shan-Fei Wang Yangyang Li Haiyan Wang Jin-Xia Liang Chun Zhu Botao Qiao 
the financial support from the National Natural Science Foundation of China(NSFC,Nos.22363001 and 21963005);the NSFC Center for Single-Atom Catalysis(No.22388102);the National Key Research and Development Program of China(No.2022YFA1503900);the Natural Science Special Foundation of Guizhou University(No.202140).
Oxide-supported metal single-atom catalysts(SACs)have exhibited excellent catalytic performance for water-gas shift(WGS)reaction.Here,we report the single-atom catalyst Pt1/FeOx exhibits excellent medium temperature c...
关键词：water-gas shift(WGS)reaction single-atom catalyst(SAC) density functional theory(DFT) thermocatalysis 
Harnessing spin effects for heterogeneous single-atom spin catalysis
《National Science Review》2024年第9期10-12,共3页Xu Han Jinxing Chen Peng He Jiong Lu 
Single-atom catalysts(SACs)are renowned for their remarkable efficiency and precise atomic utilization,offering meticulous control over the atomic environment and electronic structures of well-defined active centers.
关键词：centers. CATALYSIS PRECISE 
Single-atom catalysis for advanced oxidation and reduction systems in water decontamination
《Rare Metals》2024年第8期3576-3606,共31页Jie Teng Jin-Hui Xu Wen-Xin Sun Xue-Feng Liu Xia Xu Guo-Shuai Liu 
financially supported by the National Natural Science Foundation of China (No.52200055);the Natural Science Foundation of Jiangsu Province (No.BK20210483);China Postdoctoral Science Foundation (No.2022T150271);the Natural Science Research of Jiangsu Higher Education Institutions of China (No.23KJB610001)。
Water scarcity is an escalating global crisis,posing a severe threat to populations worldwide.Consequently,exploring various materials to remove emerging contaminants from freshwater sources has garnered significant a...
关键词：Single-atom catalysis Water treatment OXIDATION REDUCTION 
Single-atom catalysis:a promising avenue for precisely controlling reaction pathways
《Frontiers of Chemical Science and Engineering》2024年第7期97-120,共24页Xiaobo Yang Xuning Li Yanqiang Huang 
financially supported by the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB0600200);the National Key Research and Development Program of China(Grant No.2021YFA1500502);the NSFC Center for Single-Atom Catalysis(Grant No.22388102);the National Natural Science Foundation of China(Grant Nos.22102176,U19A2015 and 21925803);CAS Project for Young Scientists in Basic Research(Grant Nos.YSBR-051,YSBR-022)。
Single-atom catalysts (SACs), characterized by exceptionally high atom efficiency, have garnered significant attention across various catalytic reactions. Recent studies have showcased SACs with robust capabilities fo...
关键词：single atom catalysts selective oxidation CO_(2)RR bond coupling 
Unlocking single-atom catalysts via amorphous substrates被引量：2
《Nano Research》2024年第5期3533-3546,共14页Bohua Sun Mingyuan Xu Xiaoxia Li Baohong Zhang Rui Hao Xiaoyu Fan Binbin Jia Dingshun She 
supported by the National Natural Science Foundation of China(No.22305051);the National Key Research and Development Project(No.2023YFF0611100);the Fundamental Research Funds for the Central Universities(No.265QZ2022002);the Natural Science Foundation of Henan Province(No.232300421104);the Funding of GRIMAT Engineering Institute(No.5222201);the National Key R&D Program of China(No.2021YFB4001301-2)。
Single-atom catalysts(SACs)reveal great potential for application in catalysis due to their fully exposed active sites.In general,single atoms(SAs)and the coordination substrates need to have strong interactions or ch...
关键词：single-atoms amorphous substrate synthetic strategy CATALYSIS 
Surprised by exceptional stability of confined single-atom cluster catalysts
《Science China Materials》2024年第5期1676-1677,共2页Aiqin Wang Tao Zhang 
Single-atom catalysts(SACs)have recently grown as one of the most active frontiers in heterogeneous catalysis[1,2].Intensive research efforts have been invested towards exploring various SACs for thermocatalysis,elect...
关键词：structure CATALYSIS exceptional 
In-situ observation of structural evolution of single-atom catalysts:From synthesis to catalysis
《ChemPhysMater》2024年第1期24-35,共12页Lei Wang Shuyuan Lyu Shuohao Li 
the National Natural Science Foundation of China(52204255);Jiangsu Key Laboratory of Coal-based Greenhouse Gas Control and Utilization(PCSX202201);China Postdoctoral Science Foundation(2020M682764);the Yangzhou University Start-up Foundation.
Atomically dispersed single-atom catalysts(SACs)have been extensively studied over the past decade because of their high atom utilization efficiencies and specific selectivities.Although numerous strategies have been ...
关键词：Single-atom catalysts Structural transformation ATOMIZATION Environmental electron microscope 
Towards catalytic reactions of Cu single-atom catalysts:Recent progress and future perspective
《Chinese Chemical Letters》2024年第2期197-207,共11页Yitao Zhao Lei Tao 
financially supported by the Postgraduate Research&Practice Innovation Program of Jiangsu Province(No.KYCX21_2795);the Basic Science(Natural Science)Research Project of Colleges and Universities of Jiangsu Province(No.21KJB540001);Changzhou Sci&Tech Program(Nos.CJ20220180,CJ20210042),China.
One of the urgent and challenging topics in diversified sustainable energy conversion is the development of high-performance,low-cost,and well durable catalysts.Cu single-atom catalysts(SACs)have become promising cata...
关键词：Cu SACs Energy conversion CATALYSIS Coordination environment 
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