秋冬季节珠三角典型区域气溶胶浓度垂直分布的激光雷达反演  

Vertical distribution of aerosol mass concentration over Pearl River Delta observed by Lidar during autumn and winter

作　　者：吴仪[1] 邓孺孺[1,2,3] 秦雁 王春梅[4] 梁业恒 熊龙海[1] WU Yi;DENG Ruru;QIN Yan;WANG Chunmei;LIANG Yeheng;XIONG Longhai(School of Geographic Science and Planning,Sun Yat-sen University,Guangzhou 510275,China;Guangdong Engineering Research Center of Water Environment Remote Sensing Monitoring,Guangzhou 510275,China;Guangdong Provincial Key Laboratory of Urbanization and Geo-Simulation,Guangzhou 510275,China;School of Internet Finance and Information Engineering,Guangdong University of Finance,Guangzhou 510520,China)

机构地区：[1]中山大学地理科学与规划学院,广州510275 [2]广东省水环境遥感监测工程技术研究中心,广州510275 [3]广东省城市化与地理环境空间模拟重点实验室,广州510275 [4]广东金融学院互联网金融与信息工程学院,广州510520

出　　处：《遥感学报》2020年第3期302-318,共17页NATIONAL REMOTE SENSING BULLETIN

基　　金：国家自然科学基金(编号:41071230);广东省省级科技计划项目(编号:2017B020216001);广东省水利科技创新项目(编号:2016-08);广东省自然科学基金(编号:2017A030313238);中山大学青年教师培育项目(编号:17lgpy41);中国博士后科学基金资助项目(编号:2017M612792)。

摘　　要：气溶胶与全球热辐射平衡、水循环、人类健康密不可分,其观测精度直接影响天气预测、气候建模以及对人类健康影响评估的精度,激光雷达能监测气溶胶的垂直分布,对污染气溶胶的扩散趋势、污染源反演、气候预测等均有重要意义。本文基于激光在大气中的辐射传输过程,根据米散射激光雷达的工作原理,使用雷达的多个系统参数计算雷达常数,建立激光雷达气溶胶质量浓度反演模型,从地面向上在晴空条件下进行了珠三角地区典型区域的秋冬季节气溶胶垂直观测的实验,计算气溶胶质量浓度的垂直廓线,反演气溶胶的垂直分布情况。验证与分析结果表明:(1)激光雷达反演结果显示,白天的反演结果中噪声大大减少,表明反演算法能够有效减弱太阳光的影响。(2)相比于传统方法,使用雷达常数而非边界值的反演结果波动较小,更符合实际,能够有效避免高空噪声的影响。(3)高层大气在晴朗静稳天气状况下较为干净,气溶胶基本分布在低空区域,质量浓度随高度基本呈负指数分布。This study aims to analyze the vertical distribution of aerosol particles during autumn and winter by deriving the number density of aerosol particles from Mie Lidar return signals. Haze has always existed in regions with low humidity and stable weather. In such regions,particle vertical distribution characters are needed for transport mechanisms. As a widely used instrument, Mie Lidar surfer from the uncertainties caused by the Lidar ratio and boundary value assumption. However, Mie Lidar is the most powerful tool to observe the atmospheric vertical distribution because it performs well in day and night under all weather conditions in comparison with passive sensors.Moreover, Mie Lidar is easier to carry compared with Raman Lidar.Lidar radiation principles were studied to understand the Lidar equation and its solution. Several parameters were carefully chosen for the numerical solutions. Instead of using boundary value for approximation, the Lidar parameter k was directly calculated on the basis of Lidar-validated parameters to avoid uncertainties. Thus, aerosol particles backscatter and extinction coefficient were retrieved by solving the Lidar equation and integrated for Aerosol Optical Depth(AOD) results. A Cimel CE318 sun photometer and an ASD Field Spec3 were used to measure AOD as validation data. Lastly, the number density of aerosol particles was derived on the basis of Mie theory with the estimation of aerosol particle distribution, size, and refractive index of particles.According to the number density vertical profile, nearly no difference was observed between the number density vertical profile of aerosol particles during daytime and nighttime in one day at a low altitude. This result indicated that the sunlight effect is ignorable for aerosol particle distribution near ground. The retrieved AODs with the CE318 and ASD observations showed a root mean square error of approximately 0.0541 and 0.0100, demonstrating that the retrieved result is reliable. The comparison with traditional method showed that

关 键 词：激光雷达 辐射传输机理 气溶胶 颗粒物 质量浓度 珠三角地区 

分 类 号：X513[环境科学与工程—环境工程]