极地气溶胶及雪冰中非海盐硫酸根与甲基磺酸 时空分布及环境指示  

STUDIES ON POLAR NON-SEA-SALT SULFATE(nssSO_(4)^(2-)) AND METHANESULFONATE(MSA)AND THEIR ENVIRONMENTAL INDICATIONS

作　　者：马红梅[1] 孙波[1] 胡正毅 史贵涛 Ma Hongmei;Sun Bo;Hu Zhengyi;Shi Guitao(MNR Key Laboratory for Polar Science,Polar Research Institute of China,Shanghai 200136,China;Key Laboratory of Geographic Information Science(Ministry of Education),School of Geographic Sciences,East China Normal University,Shanghai 200241,China)

机构地区：[1]中国极地研究中心,自然资源部极地科学重点实验室,上海200136 [2]华东师范大学地理科学学院,地理信息科学教育部重点实验室,上海200241

出　　处：《极地研究》2021年第2期171-182,共12页Chinese Journal of Polar Research

基　　金：国家自然科学基金(41876225);国家自然科学基金极地专项(41941006);国家重点研发计划(2019YFC1509102)资助。

摘　　要：非海盐硫酸根(nssSO_(4)^(2-))和甲基磺酸(MSA)是极地气溶胶和雪冰介质中主要的含硫化合物。空间尺度上,南半球nssSO_(4)^(2-)和MSA具有明显的纬度效应特征;时间尺度上,nssSO_(4)^(2-)和MSA具有季节变化特征(夏高冬低),南极冰芯中MSA和nssSO_(4)^(2-)浓度均在冰期增大,北极冰芯记录出现MSA浓度在冰期减小、但是nssSO_(4)^(2-)浓度在冰期仍然增大的现象。利用极地nssSO_(4)^(2-)和MSA可以指示海洋初级生产力、大气温度、海冰范围变化以及人类活动影响等气候环境信息,并对利用nssSO_(4)^(2-)和MSA开展全球变化研究进行了展望。The main sulfur compounds of polar aerosols and snow-ice media are nssSO_(4)^(2-)and MSA.Spatially,nssSO_(4)^(2-)and MSA have obvious latitude effect characteristics.Temporally,nssSO_(4)^(2-)and MSA have interannual variation characteristics(high in summer and low in winter).The concentrations of nssSO_(4)^(2-)and MSA in Antarctic ice cores increased during glacial periods,whereas the MSA concentration of Arctic ice cores decreased during glacial periods,although the nssSO_(4)^(2-)concentration still increases during glacial periods.Both nssSO_(4)^(2-)and MSA can be used to infer climate and environmental information such as marine primary productivity,atmospheric temperature,changes in sea ice extent and human influence.The prospect of using nssSO_(4)^(2-)and MSA to study global change is also discussed.

关 键 词：nssSO_(4)^(2-) MSA 极地气溶胶 冰芯 气候环境指示 全球变化 

分 类 号：X16[环境科学与工程—环境科学] P941.6[天文地球—自然地理学] P402